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@ARTICLE{delBarrio:150729,
author = {del Barrio, Jesús and Blasco, Eva and Toprakcioglu, Chris
and Koutsioumpas, Alexandros and Scherman, Oren A. and
Oriol, Luis and Sánchez-Somolinos, Carlos},
title = {{S}elf-{A}ssembly and {P}hotoinduced {O}ptical {A}nisotropy
in {D}endronized {S}upramolecular {A}zopolymers},
journal = {Macromolecules},
volume = {47},
number = {3},
issn = {1520-5835},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2014-00775},
pages = {897–906},
year = {2014},
abstract = {Herein we report the preparation and characterization of
dendronized supramolecular polymers composed of a
carboxy-terminated azodendron, dAZO, and two different
vinylpyridine-containing polymers: poly(4-vinylpyridine)
(P4VP) and polystyrene-b-poly(4-vinylpyridine) (PS-b-P4VP)
block copolymer. P4VP can selectively complex dAZO through
hydrogen-bonding interactions, thus resulting in liquid
crystalline materials. Additionally, this strategy is also
applicable to the preparation of dendronized supramolecular
block copolymers (BCs). Lamellar, cylindrical, and spherical
morphologies are observed for the BC complexes depending on
the dAZO to vinylpyridine repeating unit ratio. Photoinduced
orientation of the azobenzene moieties is obtained in films
of the H-bonded materials—both P4VP and PS-b-P4VP based
complexes—by using 488 nm linearly polarized light and
characterized through birefringence and dichroism
measurements. High and stable values of birefringence are
obtained for polymers with azobenzene content as low as 2.7
wt $\%,$ thus demonstrating the benefits of preorganization
in photoactive dendritic moieties in side-chain H-bonded
materials.},
cin = {Neutronenstreuung ; JCNS-1 / JCNS (München) ; Jülich
Centre for Neutron Science JCNS (München) ; JCNS-FRM-II /
ICS-1},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-1-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)ICS-1-20110106},
pnm = {451 - Soft Matter Composites (POF2-451) / 54G - JCNS
(POF2-54G24)},
pid = {G:(DE-HGF)POF2-451 / G:(DE-HGF)POF2-54G24},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000331344200003},
doi = {10.1021/ma402369p},
url = {https://juser.fz-juelich.de/record/150729},
}