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@ARTICLE{Chen:150933,
author = {Chen, Lei and Küppers, Stephan and Wang, Zheng and Xiang,
Xinyi and Cao, Shiwei},
title = {{O}nline electro-{F}enton-mass spectrometry reveals
2,4′,5-trichlorobiphenyl oxidation products and binding to
organic matter},
journal = {Environmental chemistry letters},
volume = {12},
number = {2},
issn = {1610-3661},
address = {Berlin [u.a.]},
publisher = {Springer},
reportid = {FZJ-2014-00966},
pages = {329-334},
year = {2014},
abstract = {Electrochemistry–mass spectrometry is used to simulate
redox reactions in many research disciplines because this
technique is fast and provides information on compound
metabolites. However, the analysis of the degradation of
refractory organic pollutants by reactive oxygen species is
difficult to achieve by the electrochemistry step.
Therefore, here we use online electro-Fenton-mass
spectrometry to study for the first time the oxidation of
2,4′,5-trichlorobiphenyl [polychlorinated biphenyl (PCB)
31] by reactive oxygen species and the binding reactions of
PCB degradation products with model substances of natural
organic matter. The degradation products were identified by
coupled Q Trap mass spectrometry. We observed a binding of a
degradation product with γ-l-glutamyl-l-cysteinyl-glycine.
We propose a transformation pathway. We conclude that online
electro-Fenton-mass spectrometry is a promising technique to
study the oxidation of refractory organic pollutants and
further binding of degradation products with natural organic
matter.},
cin = {ZEA-3},
ddc = {540},
cid = {I:(DE-Juel1)ZEA-3-20090406},
pnm = {211 - Global Processes: Integrated Monitoring and Modelling
(POF3-211)},
pid = {G:(DE-HGF)POF3-211},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000335662000009},
doi = {10.1007/s10311-013-0447-x},
url = {https://juser.fz-juelich.de/record/150933},
}