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000151177 0247_ $$2doi$$a10.1038/nphoton.2012.261
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000151177 1001_ $$0P:(DE-HGF)0$$aRudek, Benedikt$$b0$$eCorresponding author
000151177 245__ $$aUltra-efficient ionization of heavy atoms by intense X-ray free-electron laser pulses
000151177 260__ $$aLondon [u.a.]$$bNature Publ. Group$$c2012
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000151177 520__ $$aX-ray free-electron lasers provide unique opportunities for exploring ultrafast dynamics and for imaging the structures of complex systems. Understanding the response of individual atoms to intense X-rays is essential for most free-electron laser applications. First experiments have shown that, for light atoms, the dominant interaction mechanism is ionization by sequential electron ejection, where the highest charge state produced is defined by the last ionic state that can be ionized with one photon. Here, we report an unprecedentedly high degree of ionization of xenon atoms by 1.5 keV free-electron laser pulses to charge states with ionization energies far exceeding the photon energy. Comparing ion charge-state distributions and fluorescence spectra with state-of-the-art calculations, we find that these surprisingly high charge states are created via excitation of transient resonances in highly charged ions, and predict resonance enhanced absorption to be a general phenomenon in the interaction of intense X-rays with systems containing high-Z constituents.
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000151177 7001_ $$0P:(DE-HGF)0$$aSon, Sang-Kil$$b1
000151177 7001_ $$0P:(DE-HGF)0$$aFoucar, Lutz$$b2
000151177 7001_ $$0P:(DE-HGF)0$$aEpp, Sascha W.$$b3
000151177 7001_ $$0P:(DE-HGF)0$$aErk, Benjamin$$b4
000151177 7001_ $$0P:(DE-HGF)0$$aHartmann, Robert$$b5
000151177 7001_ $$0P:(DE-HGF)0$$aAdolph, Marcus$$b6
000151177 7001_ $$0P:(DE-HGF)0$$aAndritschke, Robert$$b7
000151177 7001_ $$0P:(DE-HGF)0$$aAquila, Andrew$$b8
000151177 7001_ $$0P:(DE-HGF)0$$aBerrah, Nora$$b9
000151177 7001_ $$0P:(DE-HGF)0$$aBostedt, Christoph$$b10
000151177 7001_ $$0P:(DE-HGF)0$$aBozek, John$$b11
000151177 7001_ $$0P:(DE-HGF)0$$aCoppola, Nicola$$b12
000151177 7001_ $$0P:(DE-HGF)0$$aFilsinger, Frank$$b13
000151177 7001_ $$0P:(DE-Juel1)133892$$aGorke, Hubert$$b14$$ufzj
000151177 7001_ $$0P:(DE-HGF)0$$aGorkhover, Tais$$b15
000151177 7001_ $$0P:(DE-HGF)0$$aGraafsma, Heinz$$b16
000151177 7001_ $$0P:(DE-HGF)0$$aGumprecht, Lars$$b17
000151177 7001_ $$0P:(DE-HGF)0$$aHartmann, Andreas$$b18
000151177 7001_ $$0P:(DE-HGF)0$$aHauser, Günter$$b19
000151177 7001_ $$0P:(DE-HGF)0$$aHerrmann, Sven$$b20
000151177 7001_ $$0P:(DE-HGF)0$$aHirsemann, Helmut$$b21
000151177 7001_ $$0P:(DE-HGF)0$$aHoll, Peter$$b22
000151177 7001_ $$0P:(DE-HGF)0$$aHömke, André$$b23
000151177 7001_ $$0P:(DE-HGF)0$$aJournel, Loic$$b24
000151177 7001_ $$0P:(DE-HGF)0$$aKaiser, Christian$$b25
000151177 7001_ $$0P:(DE-HGF)0$$aKimmel, Nils$$b26
000151177 7001_ $$0P:(DE-HGF)0$$aKrasniqi, Faton$$b27
000151177 7001_ $$0P:(DE-HGF)0$$aKühnel, Kai-Uwe$$b28
000151177 7001_ $$0P:(DE-HGF)0$$aMatysek, Michael$$b29
000151177 7001_ $$0P:(DE-HGF)0$$aMesserschmidt, Marc$$b30
000151177 7001_ $$0P:(DE-HGF)0$$aMiesner, Danilo$$b31
000151177 7001_ $$0P:(DE-HGF)0$$aMöller, Thomas$$b32
000151177 7001_ $$0P:(DE-HGF)0$$aMoshammer, Robert$$b33
000151177 7001_ $$0P:(DE-HGF)0$$aNagaya, Kiyonobu$$b34
000151177 7001_ $$0P:(DE-HGF)0$$aNilsson, Björn$$b35
000151177 7001_ $$0P:(DE-HGF)0$$aPotdevin, Guillaume$$b36
000151177 7001_ $$0P:(DE-HGF)0$$aPietschner, Daniel$$b37
000151177 7001_ $$0P:(DE-HGF)0$$aReich, Christian$$b38
000151177 7001_ $$0P:(DE-HGF)0$$aRupp, Daniela$$b39
000151177 7001_ $$0P:(DE-HGF)0$$aSchaller, Gerhard$$b40
000151177 7001_ $$0P:(DE-HGF)0$$aSchlichting, Ilme$$b41
000151177 7001_ $$0P:(DE-HGF)0$$aSchmidt, Carlo$$b42
000151177 7001_ $$0P:(DE-HGF)0$$aSchopper, Florian$$b43
000151177 7001_ $$0P:(DE-HGF)0$$aSchorb, Sebastian$$b44
000151177 7001_ $$0P:(DE-HGF)0$$aSchröter, Claus-Dieter$$b45
000151177 7001_ $$0P:(DE-HGF)0$$aSchulz, Joachim$$b46
000151177 7001_ $$0P:(DE-HGF)0$$aSimon, Marc$$b47
000151177 7001_ $$0P:(DE-HGF)0$$aSoltau, Heike$$b48
000151177 7001_ $$0P:(DE-HGF)0$$aStrüder, Lothar$$b49
000151177 7001_ $$0P:(DE-HGF)0$$aUeda, Kiyoshi$$b50
000151177 7001_ $$0P:(DE-HGF)0$$aWeidenspointner, Georg$$b51
000151177 7001_ $$0P:(DE-HGF)0$$aSantra, Robin$$b52
000151177 7001_ $$0P:(DE-HGF)0$$aUllrich, Joachim$$b53
000151177 7001_ $$0P:(DE-HGF)0$$aRudenko, Artem$$b54
000151177 7001_ $$0P:(DE-HGF)0$$aRolles, Daniel$$b55
000151177 773__ $$0PERI:(DE-600)2264673-5$$a10.1038/nphoton.2012.261$$gVol. 6, no. 12, p. 858 - 865$$n12$$p858 - 865$$tNature photonics$$v6$$x1749-4893$$y2012
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