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@ARTICLE{Chapman:151178,
author = {Chapman, Henry N. and Fromme, Petra and Barty, Anton and
White, Thomas A. and Kirian, Richard A. and Aquila, Andrew
and Hunter, Mark S. and Schulz, Joachim and DePonte, Daniel
P. and Weierstall, Uwe and Doak, R. Bruce and Maia, Filipe
R. N. C. and Martin, Andrew V. and Schlichting, Ilme and
Lomb, Lukas and Coppola, Nicola and Shoeman, Robert L. and
Epp, Sascha W. and Hartmann, Robert and Rolles, Daniel and
Rudenko, Artem and Foucar, Lutz and Kimmel, Nils and
Weidenspointner, Georg and Holl, Peter and Liang, Mengning
and Barthelmess, Miriam and Caleman, Carl and Boutet,
Sébastien and Bogan, Michael J. and Krzywinski, Jacek and
Bostedt, Christoph and Bajt, Saša and Gumprecht, Lars and
Rudek, Benedikt and Erk, Benjamin and Schmidt, Carlo and
Hömke, André and Reich, Christian and Pietschner, Daniel
and Strüder, Lothar and Hauser, Günter and Gorke, Hubert
and Ullrich, Joachim and Herrmann, Sven and Schaller,
Gerhard and Schopper, Florian and Soltau, Heike and Kühnel,
Kai-Uwe and Messerschmidt, Marc and Bozek, John D. and
Hau-Riege, Stefan P. and Frank, Matthias and Hampton,
Christina Y. and Sierra, Raymond G. and Starodub, Dmitri and
Williams, Garth J. and Hajdu, Janos and Timneanu, Nicusor
and Seibert, M. Marvin and Andreasson, Jakob and Rocker,
Andrea and Jönsson, Olof and Svenda, Martin and Stern,
Stephan and Nass, Karol and Andritschke, Robert and
Schröter, Claus-Dieter and Krasniqi, Faton and Bott, Mario
and Schmidt, Kevin E. and Wang, Xiaoyu and Grotjohann, Ingo
and Holton, James M. and Barends, Thomas R. M. and Neutze,
Richard and Marchesini, Stefano and Fromme, Raimund and
Schorb, Sebastian and Rupp, Daniela and Adolph, Marcus and
Gorkhover, Tais and Andersson, Inger and Hirsemann, Helmut
and Potdevin, Guillaume and Graafsma, Heinz and Nilsson,
Björn and Spence, John C. H.},
title = {{F}emtosecond {X}-ray protein nanocrystallography},
journal = {Nature},
volume = {470},
number = {7332},
issn = {1476-4687},
address = {London [u.a.]},
publisher = {Nature Publising Group},
reportid = {FZJ-2014-01177},
pages = {73 - 77},
year = {2011},
abstract = {X-ray crystallography provides the vast majority of
macromolecular structures, but the success of the method
relies on growing crystals of sufficient size. In
conventional measurements, the necessary increase in X-ray
dose to record data from crystals that are too small leads
to extensive damage before a diffraction signal can be
recorded1, 2, 3. It is particularly challenging to obtain
large, well-diffracting crystals of membrane proteins, for
which fewer than 300 unique structures have been determined
despite their importance in all living cells. Here we
present a method for structure determination where
single-crystal X-ray diffraction ‘snapshots’ are
collected from a fully hydrated stream of nanocrystals using
femtosecond pulses from a hard-X-ray free-electron laser,
the Linac Coherent Light Source4. We prove this concept with
nanocrystals of photosystem I, one of the largest membrane
protein complexes5. More than 3,000,000 diffraction patterns
were collected in this study, and a three-dimensional data
set was assembled from individual photosystem I nanocrystals
(~200 nm to 2 μm in size). We mitigate the problem of
radiation damage in crystallography by using pulses briefer
than the timescale of most damage processes6. This offers a
new approach to structure determination of macromolecules
that do not yield crystals of sufficient size for studies
using conventional radiation sources or are particularly
sensitive to radiation damage.},
cin = {ZEA-2},
ddc = {070},
cid = {I:(DE-Juel1)ZEA-2-20090406},
pnm = {531 - Hadron Structure and Dynamics (HSD) (POF2-531)},
pid = {G:(DE-HGF)POF2-531},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000286886400036},
pubmed = {pmid:21293373},
doi = {10.1038/nature09750},
url = {https://juser.fz-juelich.de/record/151178},
}