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@ARTICLE{Voigt:15134,
author = {Voigt, C. and Schumann, U. and Jurkat, T. and Schäuble, D.
and Schlager, H. and petzold, A. and Gayet, J.F. and
Krämer, M. and Schneider, J. and Borrmann, S. and Schmale,
J. and Jessberger, P. and Hamburger, T. and Lichenstern, M.
and Scheibe, M. and Gourbeyre, C. and Meyer, J. and
Kübbeler, M. and Frey, W. and Kalesse, H. and Butler, K.
and Lawrence, M.G. and Holzäpfle, F. and Arnold, F. and
Wendisch, M. and Döpelheuer, A. and Gotsschaldt, K. and
Baumann, R. and Zöger, M. and Sölch, I. and Rautenhaus, M.
and Dörnbrack, A.},
title = {{I}n-situ observations of young contails overview and
selected results from the {CONCERT} campagin},
journal = {Atmospheric chemistry and physics},
volume = {10},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-15134},
pages = {9039 - 9056},
year = {2010},
note = {The CONCERT campaign was organized by the HGF-junior
research group AEROTROP (Impact of Aircraft Emissions on the
heteROgeneous chemistry of the TROPopause region). Part of
this work was funded within the DLR-project CATS
(Climate-compatible Air Transport System) and by the DFG SPP
HALO 1294. We thank the DLR flight department for their
excellent support during the campaign. A. Giez is greatfully
acknowledged for his help with the calibration of the
dewpoint hygrometer. ECMWF forecasts were provided in the
context of the ECMWF Special Project: Support Tool for HALO
Missions.},
abstract = {Lineshaped contrails were detected with the research
aircraft Falcon during the CONCERT - CONtrail and Cirrus
ExpeRimenT - campaign in October/November 2008. The Falcon
was equipped with a set of instruments to measure the
particle size distribution, shape, extinction and chemical
composition as well as trace gas mixing ratios of sulfur
dioxide (SO2), reactive nitrogen and halogen species (NO,
NOy, HNO3, HONO, HCl), ozone (O-3) and carbon monoxide (CO).
During 12 mission flights over Europe, numerous contrails,
cirrus clouds and a volcanic aerosol layer were probed at
altitudes between 8.5 and 11.6 km and at temperatures above
213 K. 22 contrails from 11 different aircraft were observed
near and below ice saturation. The observed NO mixing
ratios, ice crystal and soot number densities are compared
to a process based contrail model. On 19 November 2008 the
contrail from a CRJ-2 aircraft was penetrated in 10.1 km
altitude at a temperature of 221 K. The contrail had mean
ice crystal number densities of 125 cm(-3) with effective
radii r(eff) of 2.6 mu m. The presence of particles with r >
50 mu m in the less than 2 min old contrail suggests that
natural cirrus crystals were entrained in the contrail. Mean
HONO/NO (HONO/NOy) ratios of 0.037 (0.024) and the fuel
sulfur conversion efficiency to H2SO4 (epsilon(S)down arrow)
of $2.9\%$ observed in the CRJ-2 contrail are in the range
of previous measurements in the gaseous aircraft exhaust. On
31 October 2010 aviation NO emissions could have contributed
by more than $40\%$ to the regional scale NO levels in the
mid-latitude lowest stratosphere. The CONCERT observations
help to better quantify the climate impact from contrails
and will be used to investigate the chemical processing of
trace gases on contrails.},
keywords = {J (WoSType)},
cin = {IEK-7},
ddc = {550},
cid = {I:(DE-Juel1)IEK-7-20101013},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK491},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000282429000023},
doi = {10.5194/acp-10-9039-2010},
url = {https://juser.fz-juelich.de/record/15134},
}