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@ARTICLE{Fry:15262,
      author       = {Fry, J.L. and Kiendler-Scharr, A. and Rollins, A.W. and
                      Brauers, T. and Brown, S.S. and Dorn, H.-P. and Dubé, W.P.
                      and Fuchs, H. and Mensah, A. and Rohrer, F. and Tillmann, R.
                      and Wahner, A. and Woolridge, P.J. and Cohen, R.C.},
      title        = {{SOA} from limonene: role of {NO}3 in its generation and
                      degradation},
      journal      = {Atmospheric chemistry and physics},
      volume       = {11},
      issn         = {1680-7316},
      address      = {Katlenburg-Lindau},
      publisher    = {EGU},
      reportid     = {PreJuSER-15262},
      pages        = {3879 - 3894},
      year         = {2011},
      note         = {The Berkeley authors were supported by NSF ATM-0639847 and
                      NSF ATM-0511829. The authors thank the entire SAPHIR
                      NO<INF>3</INF> intercomparison campaign team, June 2007 at
                      Forschungszentrum Julich, for their support of these
                      experiments. This work was a joint activity of the European
                      Network of Excellence ACCENT (contract no: GOCE
                      CT-2004-505337) and EUROCHAMP.},
      abstract     = {The formation of organic nitrates and secondary organic
                      aerosol (SOA) were monitored during the NO3 + limonene
                      reaction in the atmosphere simulation chamber SAPHIR at
                      Research Center Julich. The 24-h run began in a purged, dry,
                      particle-free chamber and comprised two injections of
                      limonene and oxidants, such that the first experiment
                      measured SOA yield in the absence of seed aerosol, and the
                      second experiment yields in the presence of 10 mu g m(-3)
                      seed organic aerosol. After each injection, two separate
                      increases in aerosol mass were observed, corresponding to
                      sequential oxidation of the two limonene double bonds.
                      Analysis of the measured NO3, limonene, product nitrate
                      concentrations, and aerosol properties provides mechanistic
                      insight and constrains rate constants, branching ratios and
                      vapor pressures of the products. The organic nitrate yield
                      from NO3 + limonene is approximate to $30\%.$ The SOA mass
                      yield was observed to be $25-40\%.$ The first injection is
                      reproduced by a kinetic model. PMF analysis of the aerosol
                      composition suggests that much of the aerosol mass results
                      from combined oxidation by both O-3 and NO3, e. g.,
                      oxidation of NO3 + limonene products by O-3. Further, later
                      aerosol nitrate mass seems to derive from heterogeneous
                      uptake of NO3 onto unreacted aerosol alkene.},
      keywords     = {J (WoSType)},
      cin          = {IEK-8},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {Atmosphäre und Klima},
      pid          = {G:(DE-Juel1)FUEK491},
      shelfmark    = {Meteorology $\&$ Atmospheric Sciences},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000290014300022},
      doi          = {10.5194/acp-11-3879-2011},
      url          = {https://juser.fz-juelich.de/record/15262},
}