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000015284 084__ $$2WoS$$aChemistry, Physical
000015284 1001_ $$0P:(DE-HGF)0$$aDavaasambuu, J.$$b0
000015284 245__ $$aPhase Behaviour of CoC12-MnC12 Mixed Crystals
000015284 260__ $$aMünchen$$bOldenbourg$$c2011
000015284 300__ $$a413 - 420
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000015284 440_0 $$06031$$aZeitschrift für physikalische Chemie$$v225$$x0942-9352$$y4
000015284 500__ $$aThis work was supported by the DFG under grant EC 153/3-1.
000015284 520__ $$aThermal properties of CoCl2, MnCl2 and their mixed crystals are investigated by means of temperature dependent neutron powder diffraction and time-resolved small angle neutron scattering. The coefficients of thermal expansion of these crystals have been determined as a function of temperature. The temperature-induced structural variations can be explained by distortions of CoCl5/MnCl6 octahedra and changes in Co/Mn-Cl bond lengths. CoCl2 and MnCl2 form homogeneous solid solutions in the entire temperature range between the solidus and 50 K. There is no indication of any miscibility gap as predicted from thermodynamic calculations.
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000015284 65320 $$2Author$$aMixed Crystal
000015284 65320 $$2Author$$aDemixing
000015284 65320 $$2Author$$aPhase Diagram
000015284 65320 $$2Author$$aNeutron Diffraction
000015284 65320 $$2Author$$aNeutron Small Angle Scattering
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000015284 7001_ $$0P:(DE-HGF)0$$aGüthoff, F.$$b1
000015284 7001_ $$0P:(DE-HGF)0$$aHoelzel, M.$$b2
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