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@ARTICLE{Krause:153657,
      author       = {Krause, Kay and Kätelhön, Enno and Offenhäusser, Andreas
                      and Wolfrum, Bernhard},
      title        = {{S}imulation of the impact of reversible adsorption on the
                      response time of interdigitated electrode arrays},
      journal      = {Physica status solidi / A},
      volume       = {211},
      number       = {6},
      issn         = {1862-6300},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2014-03161},
      pages        = {1352–1356},
      year         = {2014},
      abstract     = {We simulate the amperometric response time of an
                      interdigitated electrode array with respect to reversible
                      adsorption of redox active molecules at the electrode
                      surface. When neighboring electrodes are biased to
                      potentials below and above the redox potential of the
                      species under investigation, molecules can participate in
                      repetitive reactions leading to an amplification of the
                      Faradaic current. During collisions between molecules and
                      electrodes, the molecules may undergo reversible adsorption.
                      We simulate the behavior of this redox cycling process by
                      using a discrete random walk model, which mimics the
                      diffusive pathway of the molecules. Adsorption probabilities
                      are implemented via the boundary conditions at the
                      electrodes. Using this simulation, we investigate the effect
                      of reversible adsorption on the response time of the
                      interdigitated electrode array.},
      cin          = {PGI-8 / JARA-FIT},
      ddc          = {530},
      cid          = {I:(DE-Juel1)PGI-8-20110106 / $I:(DE-82)080009_20140620$},
      pnm          = {423 - Sensorics and bioinspired systems (POF2-423)},
      pid          = {G:(DE-HGF)POF2-423},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000337759000023},
      doi          = {10.1002/pssa.201330361},
      url          = {https://juser.fz-juelich.de/record/153657},
}