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000153751 005__ 20210129213801.0
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000153751 0247_ $$2ISSN$$a1866-1793
000153751 037__ $$aFZJ-2014-03240
000153751 041__ $$aEnglish
000153751 1001_ $$0P:(DE-Juel1)129535$$aSittig, Stephan$$b0$$eCorresponding Author$$gmale$$ufzj
000153751 245__ $$aSorption, Transformation and Transport of Sulfadiazine in a loess and sandy oil$$f2012-03-31
000153751 260__ $$aJülich$$bForschungszentrum Jülich GmbH Zentralbibliothek, Verlag$$c2014
000153751 300__ $$av, 121 S.
000153751 3367_ $$0PUB:(DE-HGF)11$$2PUB:(DE-HGF)$$aDissertation / PhD Thesis$$bphd$$mphd$$s153751
000153751 3367_ $$02$$2EndNote$$aThesis
000153751 3367_ $$2DRIVER$$adoctoralThesis
000153751 3367_ $$2BibTeX$$aPHDTHESIS
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000153751 3367_ $$2ORCID$$aDISSERTATION
000153751 4900_ $$aSchriften des Forschungszentrums Jülich Reihe Energie & Umwelt / Energy & Environment$$v225
000153751 502__ $$aUniversität Bonn, Diss., 2014$$bDr.$$cUniversität Bonn$$d2014
000153751 520__ $$aVeterinary antibiotics are unintentionally introduced into the environmentand therefore found in ground and surface water, soil andsediments, air, plants etc. They enter these compartments mainly via application of manure or sewage sludge to soils for fertilizing purposes or after application in aquaculture, in form of the parent compound or a transformation product. Generally, sorption, transformation and transport determines the fate of these organic contaminants in soil. Their wide-spread distribution bears several risks, i. e. spreading of resistance genes or occurrence in the foodchain. Long-term (60 days) batch studies were conducted applying radiolabelled sulfadiazine to samples from two agricultural soils to investigate the sorption and sequestration behavior in the plow layers. Sequential extractions at several time-steps served to analyze the dynamics of both processes. A numerical evaluation served to describe instantaneous sorption, the dynamics of sorption and sequestration, and the formation of non-extractable residues. Multiple extractions with the harsh method questioned the concept of non-extractable residues, since with each consecutive extraction step, further sulfadiazine could be extracted. Analyzing the liquid phase and the extracts from these batch experiments with Radio-HPLC served to improve the understanding of the transformation behavior in soils in different degrees of (bio-)availability. Apart from the deduction of rate-parameters for acompartment model, the resemblance of the compositions in the liquid phases and the harsh extracts was demonstrated. The formation of the up to six transformation products showed distinct dynamics, either spontaneous or with a time-lag. ...
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000153751 773__ $$y2014
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000153751 9132_ $$0G:(DE-HGF)POF3-255$$1G:(DE-HGF)POF3-250$$2G:(DE-HGF)POF3-200$$aDE-HGF$$bPOF III$$lMarine, Küsten- und Polare Systeme$$vTerrestrische Umwelt$$x0
000153751 9131_ $$0G:(DE-HGF)POF2-246$$1G:(DE-HGF)POF2-240$$2G:(DE-HGF)POF2-200$$3G:(DE-HGF)POF2$$4G:(DE-HGF)POF$$aDE-HGF$$bErde und Umwelt$$lTerrestrische Umwelt$$vModelling and Monitoring Terrestrial Systems: Methods and Technologies$$x0
000153751 9131_ $$0G:(DE-HGF)POF3-255$$1G:(DE-HGF)POF3-250$$2G:(DE-HGF)POF3-200$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF3-255$$aDE-HGF$$bErde und Umwelt$$lTerrestrische Umwelt$$vTerrestrial Systems: From Observation to Prediction$$x1
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