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@ARTICLE{Kang:153767,
      author       = {Kang, Kyongok},
      title        = {{G}lass transition of repulsive charged rods (fd-viruses)},
      journal      = {Soft matter},
      volume       = {10},
      number       = {18},
      issn         = {1744-6848},
      address      = {Cambridge},
      publisher    = {Royal Society of Chemistry (RSC)},
      reportid     = {FZJ-2014-03256},
      pages        = {3311 - 3324},
      year         = {2014},
      abstract     = {It has recently been shown that suspensions of long and
                      thin charged fibrous viruses (fd) form a glass at low ionic
                      strengths. The corresponding thick electric double layers
                      give rise to long-ranged repulsive electrostatic
                      interactions, which lead to caging and structural arrest at
                      concentrations far above the isotropic–nematic coexistence
                      region. Structural arrest and freezing of the orientational
                      texture are found to occur at the same concentration. In
                      addition, various types of orientational textures are
                      equilibrated below the glass transition concentration,
                      ranging from a chiral-nematic texture with a large pitch (of
                      about 100 μm), an X-pattern, and a tightly packed domain
                      texture, consisting of helical domains with a relatively
                      small pitch (of about 10 μm) and twisted boundaries. The
                      dynamics of both particles as well as the texture are
                      discussed, below and above the glass transition. Dynamic
                      light scattering correlation functions exhibit two dynamical
                      modes, where the slow mode is attributed to the elasticity
                      of helical domains. On approach of the glass-transition
                      concentration, the slow mode increases in amplitude, while
                      as the amplitudes of the fast and slow mode become equal at
                      the glass transition. Finally, interesting features of the
                      “transient” behaviors of charged fd-rod glass are shown
                      as the initial caging due to structural arrest, the
                      propagation of flow originating from stress release, and the
                      transition to the final metastable glass state. In addition
                      to the intensity correlation function, power spectra are
                      presented as a function of the waiting time, at the
                      zero-frequency limit that may access to the thermal
                      anomalities in a charged system.},
      cin          = {ICS-3},
      ddc          = {530},
      cid          = {I:(DE-Juel1)ICS-3-20110106},
      pnm          = {451 - Soft Matter Composites (POF2-451)},
      pid          = {G:(DE-HGF)POF2-451},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000334685800020},
      pubmed       = {pmid:24637952},
      doi          = {10.1039/c3sm53131g},
      url          = {https://juser.fz-juelich.de/record/153767},
}