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@ARTICLE{Chihaia:153772,
author = {Chihaia, Viorel and Munteanu, Cornel and Scurtu, Rares and
Palade, Petru},
title = {{T}heoretical study of the reaction of {L}i{BH}4 with
{M}g{H}2 in presence of carbon substrate},
journal = {Revue roumaine de chimie},
volume = {57},
number = {4-5},
issn = {0035-3930},
address = {Bucuresti},
publisher = {Ed. Acad. Romane},
reportid = {FZJ-2014-03261},
pages = {435-442},
year = {2012},
abstract = {In this work we design some atomic scale simulation methods
as investigative tools in the study of the formation of
compounds for the reversible storage of hydrogen in bulk
materials. It was verified that the reaction between the
LiBH 4 and MgH 2 is energetically favored for temperatures
above 280 K and that this system can be used in the hydrogen
storage and the fuel cell application. To identify the
reaction mechanism at the interface of LiBH 4 , MgH 2 and
carbon layers we did some Molecular Dynamics simulations and
QM/MM calculations. The results show that the layers of ions
formed at the interface with the graphite may assure the
right arrangement of the atoms to start the formation of the
crystals. Moreover, the presence of the hexagonal layers of
graphite may play a role as a pattern template for the
layers of boron atoms in the MgB 2 lattice.},
cin = {JSC},
ddc = {540},
cid = {I:(DE-Juel1)JSC-20090406},
pnm = {411 - Computational Science and Mathematical Methods
(POF2-411)},
pid = {G:(DE-HGF)POF2-411},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000320072000020},
url = {https://juser.fz-juelich.de/record/153772},
}