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000154037 0247_ $$2doi$$a10.1007/12_2012_183
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000154037 1001_ $$0P:(DE-Juel1)131039$$aWinkler, Roland G.$$b0$$eCorresponding Author$$ufzj
000154037 245__ $$aStrong and Weak Polyelectrolyte Adsorption onto Oppositely Charged Curved Surfaces
000154037 260__ $$aBerlin$$bSpringer$$c2014
000154037 29510 $$aPolyelectrolyte Complexes in the Dispersed and Solid State I
000154037 300__ $$a1-56
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000154037 520__ $$aPolyelectrolytes are macromolecules composed of charged monomers and exhibit unique properties due to the interplay of their flexibility and electrostatic interactions. In solution, they are attracted to oppositely charged surfaces and interfaces and exhibit a transition to an adsorbed state when certain conditions are met concerning the charge densities of the polymer and surface and the properties of the solution. In this review, we discuss two limiting cases for adsorption of flexible polyelectrolytes on curved surfaces: weak and strong adsorption. In the first case, adsorption is strongly influenced by the entropic degrees of freedom of a flexible polyelectrolyte. By contrast, in the strong adsorption limit, electrostatic interactions dominate, which leads to particular adsorption patterns, specifically on spherical surfaces. We discuss the corresponding theoretical approaches, applying a mean-field description for the polymer and the polymer–surface interaction. For weak adsorption, we discuss the critical adsorption behavior by exactly solvable models for planar and spherical geometries and a generic approximation scheme, which is additionally applied to cylindrical surfaces. For strong adsorption, we investigate various polyelectrolyte patterns on cylinders and spheres and evaluate their stability. The results are discussed in the light of experimental results, mostly of DNA adsorption experiments
000154037 536__ $$0G:(DE-HGF)POF2-451$$a451 - Soft Matter Composites (POF2-451)$$cPOF2-451$$fPOF II$$x0
000154037 7001_ $$0P:(DE-Juel1)130595$$aCherstvy, Andrey$$b1$$ufzj
000154037 773__ $$0PERI:(DE-600)1481539-4$$a10.1007/12_2012_183$$p1-56$$tAdvances in polymer science$$v255$$x1436-5030$$y2014
000154037 8564_ $$uhttps://juser.fz-juelich.de/record/154037/files/FZJ-2014-03451.pdf$$yRestricted$$zPublished final document.
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000154037 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)131039$$aForschungszentrum Jülich GmbH$$b0$$kFZJ
000154037 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130595$$aForschungszentrum Jülich GmbH$$b1$$kFZJ
000154037 9132_ $$0G:(DE-HGF)POF3-551$$1G:(DE-HGF)POF3-550$$2G:(DE-HGF)POF3-500$$aDE-HGF$$bKey Technologies$$lBioSoft  Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences$$vFunctional Macromolecules and Complexes$$x0
000154037 9131_ $$0G:(DE-HGF)POF2-451$$1G:(DE-HGF)POF2-450$$2G:(DE-HGF)POF2-400$$3G:(DE-HGF)POF2$$4G:(DE-HGF)POF$$aDE-HGF$$bSchlüsseltechnologien$$lBioSoft$$vSoft Matter Composites$$x0
000154037 9201_ $$0I:(DE-Juel1)IAS-2-20090406$$kIAS-2$$lTheorie der Weichen Materie und Biophysik $$x0
000154037 9201_ $$0I:(DE-Juel1)ICS-2-20110106$$kICS-2$$lTheorie der Weichen Materie und Biophysik $$x1
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