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@ARTICLE{Pabst:154315,
author = {Pabst, Michael},
title = {{A}nalytical solution of the {P}oisson-{N}ernst-{P}lanck
equations for an electrochemical system close to
electroneutrality},
journal = {The journal of chemical physics},
volume = {140},
number = {22},
issn = {1089-7690},
address = {Melville, NY},
publisher = {American Institute of Physics},
reportid = {FZJ-2014-03663},
pages = {224113},
year = {2014},
abstract = {Single charge densities and the potential are used to
describe models of electrochemical systems. These quantities
can be calculated by solving a system of time dependent
nonlinear coupled partial differential equations, the
Poisson-Nernst-Planck equations. Assuming small deviations
from the electroneutral equilibrium, the linearized and
decoupled equations are solved for a radial symmetric
geometry, which represents the interface between a cell and
a sensor device. The densities and the potential are
expressed by Fourier-Bessels series. The system considered
has a ratio between the Debye-length and its geometric
dimension on the order of 10−4 so the Fourier-Bessel
series can be approximated by elementary functions. The time
development of the system is characterized by two time
constants, τ c and τ g . The constant τ c describes the
approach to the stationary state of the total charge and the
potential. τ c is several orders of magnitude smaller than
the geometry-dependent constant τ g , which is on the order
of 10 ms characterizing the transition to the stationary
state of the single ion densities.},
cin = {ICS-8},
ddc = {540},
cid = {I:(DE-Juel1)ICS-8-20110106},
pnm = {453 - Physics of the Cell (POF2-453)},
pid = {G:(DE-HGF)POF2-453},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000337806100016},
doi = {10.1063/1.4881599},
url = {https://juser.fz-juelich.de/record/154315},
}