000155387 001__ 155387
000155387 005__ 20240712101045.0
000155387 0247_ $$2doi$$a10.5194/acp-14-5327-2014
000155387 0247_ $$2ISSN$$a1680-7316
000155387 0247_ $$2ISSN$$a1680-7324
000155387 0247_ $$2Handle$$a2128/7902
000155387 0247_ $$2Handle$$a2128/7947
000155387 0247_ $$2WOS$$aWOS:000337803100005
000155387 037__ $$aFZJ-2014-04556
000155387 082__ $$a550
000155387 1001_ $$0P:(DE-HGF)0$$aTian, J.$$b0
000155387 245__ $$aModeling the evolution of aerosol particles in a ship plume using PartMC-MOSAIC
000155387 260__ $$aKatlenburg-Lindau$$bEGU$$c2014
000155387 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s155387
000155387 3367_ $$2DataCite$$aOutput Types/Journal article
000155387 3367_ $$00$$2EndNote$$aJournal Article
000155387 3367_ $$2BibTeX$$aARTICLE
000155387 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000155387 3367_ $$2DRIVER$$aarticle
000155387 520__ $$aThis study investigates the evolution of ship-emitted aerosol particles using the stochastic particle-resolved model PartMC-MOSAIC (Particle Monte Carlo model-Model for Simulating Aerosol Interactions and Chemistry). Comparisons of our results with observations from the QUANTIFY (Quantifying the Climate Impact of Global and European Transport Systems) study in 2007 in the English Channel and the Gulf of Biscay showed that the model was able to reproduce the observed evolution of total number concentration and the vanishing of the nucleation mode consisting of sulfate particles. Further process analysis revealed that during the first hour after emission, dilution reduced the total number concentration by four orders of magnitude, while coagulation reduced it by an additional order of magnitude. Neglecting coagulation resulted in an overprediction of more than one order of magnitude in the number concentration of particles smaller than 40 nm at a plume age of 100 s. Coagulation also significantly altered the mixing state of the particles, leading to a continuum of internal mixtures of sulfate and black carbon. The impact on cloud condensation nuclei (CCN) concentrations depended on the supersaturation threshold S at which CCN activity was evaluated. For the base case conditions, characterized by a low formation rate of secondary aerosol species, neglecting coagulation, but simulating condensation, led to an underestimation of CCN concentrations of about 37% for S = 0.3% at the end of the 14-h simulation. In contrast, for supersaturations higher than 0.7%, neglecting coagulation resulted in an overestimation of CCN concentration, about 75% for S = 1%. For S lower than 0.2% the differences between simulations including coagulation and neglecting coagulation were negligible. Neglecting condensation, but simulating coagulation did not impact the CCN concentrations below 0.2% and resulted in an underestimation of CCN concentrations for larger supersaturations, e.g., 18% for S = 0.6%. We also explored the role of nucleation for the CCN concentrations in the ship plume. For the base case the impact of nucleation on CCN concentrations was limited, but for a sensitivity case with higher formation rates of secondary aerosol over several hours, the CCN concentrations increased by an order of magnitude for supersaturation thresholds above 0.3%.
000155387 536__ $$0G:(DE-HGF)POF2-233$$a233 - Trace gas and aerosol processes in the troposphere (POF2-233)$$cPOF2-233$$fPOF II$$x0
000155387 588__ $$aDataset connected to CrossRef, juser.fz-juelich.de
000155387 7001_ $$0P:(DE-HGF)0$$aRiemer, N.$$b1$$eCorresponding Author
000155387 7001_ $$0P:(DE-HGF)0$$aWest, M.$$b2
000155387 7001_ $$0P:(DE-HGF)0$$aPfaffenberger, L.$$b3
000155387 7001_ $$0P:(DE-HGF)0$$aSchlager, H.$$b4
000155387 7001_ $$0P:(DE-Juel1)136669$$aPetzold, A.$$b5$$ufzj
000155387 773__ $$0PERI:(DE-600)2069847-1$$a10.5194/acp-14-5327-2014$$gVol. 14, no. 11, p. 5327 - 5347$$n11$$p5327 - 5347$$tAtmospheric chemistry and physics$$v14$$x1680-7324$$y2014
000155387 8564_ $$uhttp://www.atmos-chem-phys.net/14/5327/2014/
000155387 8564_ $$uhttps://juser.fz-juelich.de/record/155387/files/FZJ-2014-04556.pdf$$yOpenAccess
000155387 8564_ $$uhttps://juser.fz-juelich.de/record/155387/files/FZJ-2014-04556.jpg?subformat=icon-144$$xicon-144$$yOpenAccess
000155387 8564_ $$uhttps://juser.fz-juelich.de/record/155387/files/FZJ-2014-04556.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000155387 8564_ $$uhttps://juser.fz-juelich.de/record/155387/files/FZJ-2014-04556.jpg?subformat=icon-640$$xicon-640$$yOpenAccess
000155387 909CO $$ooai:juser.fz-juelich.de:155387$$pdnbdelivery$$pVDB$$pVDB:Earth_Environment$$pdriver$$popen_access$$popenaire
000155387 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)136669$$aForschungszentrum Jülich GmbH$$b5$$kFZJ
000155387 9132_ $$0G:(DE-HGF)POF3-243$$1G:(DE-HGF)POF3-240$$2G:(DE-HGF)POF3-200$$aDE-HGF$$bMarine, Küsten- und Polare Systeme$$lAtmosphäre und Klima$$vTropospheric trace substances and their transformation processes$$x0
000155387 9131_ $$0G:(DE-HGF)POF2-233$$1G:(DE-HGF)POF2-230$$2G:(DE-HGF)POF2-200$$3G:(DE-HGF)POF2$$4G:(DE-HGF)POF$$aDE-HGF$$bErde und Umwelt$$lAtmosphäre und Klima$$vTrace gas and aerosol processes in the troposphere$$x0
000155387 9141_ $$y2014
000155387 915__ $$0LIC:(DE-HGF)CCBY3$$2HGFVOC$$aCreative Commons Attribution CC BY 3.0
000155387 915__ $$0StatID:(DE-HGF)0010$$2StatID$$aJCR/ISI refereed
000155387 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR
000155387 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000155387 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000155387 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000155387 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List
000155387 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000155387 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000155387 915__ $$0StatID:(DE-HGF)0500$$2StatID$$aDBCoverage$$bDOAJ
000155387 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000155387 915__ $$0StatID:(DE-HGF)1020$$2StatID$$aDBCoverage$$bCurrent Contents - Social and Behavioral Sciences
000155387 920__ $$lyes
000155387 9201_ $$0I:(DE-Juel1)IEK-8-20101013$$kIEK-8$$lTroposphäre$$x0
000155387 9801_ $$aFullTexts
000155387 980__ $$ajournal
000155387 980__ $$aVDB
000155387 980__ $$aUNRESTRICTED
000155387 980__ $$aFullTexts
000155387 980__ $$aI:(DE-Juel1)IEK-8-20101013
000155387 981__ $$aI:(DE-Juel1)ICE-3-20101013