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@ARTICLE{Krause:155452,
author = {Krause, Christina and Zorn, Reiner and Frick, Bernhard and
Schönhals, Andreas},
title = {{T}hermal properties and vibrational density of states of a
nanoconfined discotic liquid crystal},
journal = {Colloid $\&$ polymer science},
volume = {292},
number = {8},
issn = {1435-1536},
address = {Berlin},
publisher = {Springer},
reportid = {FZJ-2014-04618},
pages = {1949 - 1960},
year = {2014},
abstract = {Neutron scattering is employed to investigate the
vibrational density of states (VDOS) of the discotic liquid
crystal 2,3,6,7,10,11-hexakis[hexyloxy] triphenylene (HAT6)
confined to the pores of alumina oxide membranes with
different pore sizes. Additionally, the phase transitions
were studied by differential scanning calorimetry. The
transitions were observed down to the smallest pore size.
The decrease of the transition enthalpies versus inverse
pore size for both transitions implies an increase of the
amount of disordered amorphous material. By extrapolation of
its pore size dependence, a critical pore diameter for
structure formation of 17 nm is estimated. Similar to the
bulk, excess contributions to the VDOS (Boson peak) are also
observed for confined HAT6. The Boson peak gains in
intensity and shifts to lower frequencies with decreasing
pore diameter. This is discussed in the framework of a
softening of HAT6 induced by the confinement due to a
less-developed plastic crystalline state inside the pores
compared to the bulk.},
cin = {ICS-1 / Neutronenstreuung ; JCNS-1},
ddc = {540},
cid = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106},
pnm = {451 - Soft Matter Composites (POF2-451) / 54G - JCNS
(POF2-54G24)},
pid = {G:(DE-HGF)POF2-451 / G:(DE-HGF)POF2-54G24},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000339888900021},
doi = {10.1007/s00396-014-3247-3},
url = {https://juser.fz-juelich.de/record/155452},
}