% IMPORTANT: The following is UTF-8 encoded.  This means that in the presence
% of non-ASCII characters, it will not work with BibTeX 0.99 or older.
% Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or
% “biber”.

@ARTICLE{Chua:155453,
      author       = {Chua, Yeong Zen and Schulz, Gunnar and Shoifet, Evgeni and
                      Huth, Heiko and Zorn, Reiner and Scmelzer, Jürn W. P. and
                      Schick, Christoph},
      title        = {{G}lass transition cooperativity from broad band heat
                      capacity spectroscopy},
      journal      = {Colloid $\&$ polymer science},
      volume       = {292},
      number       = {8},
      issn         = {1435-1536},
      address      = {Berlin},
      publisher    = {Springer},
      reportid     = {FZJ-2014-04619},
      pages        = {1893 - 1904},
      year         = {2014},
      abstract     = {Molecular dynamics is often studied by broad band
                      dielectric spectroscopy (BDS) because of the wide dynamic
                      range available and the large number of processes resulting
                      in electrical dipole fluctuations and with that in a
                      dielectrically detectable relaxation process. Calorimetry on
                      the other hand is an effective analytical tool to
                      characterize phase and glass transitions by its signatures
                      in heat capacity. In the linear response scheme, heat
                      capacity is considered as entropy compliance. Consequently,
                      only processes significantly contributing to entropy
                      fluctuations appear in calorimetric curves. The glass
                      relaxation is a prominent example for such a process. Here,
                      we present complex heat capacity at the dynamic glass
                      transition (segmental relaxation) of polystyrene (PS) and
                      poly(methyl methacrylate) (PMMA) in a dynamic range of 11
                      orders of magnitude, which is comparable to BDS. As one of
                      the results, we determined the characteristic length scale
                      of the corresponding fluctuations. The dynamic glass
                      transition measured by calorimetry is finally compared to
                      the cooling rate dependence of fictive temperature and BDS
                      data. For PS, dielectric and calorimetric data are similar
                      but for PMMA with its very strong secondary relaxation
                      process some peculiarities are observed.},
      cin          = {ICS-1 / Neutronenstreuung ; JCNS-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {451 - Soft Matter Composites (POF2-451) / 54G - JCNS
                      (POF2-54G24)},
      pid          = {G:(DE-HGF)POF2-451 / G:(DE-HGF)POF2-54G24},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000339888900015},
      doi          = {10.1007/s00396-014-3280-2},
      url          = {https://juser.fz-juelich.de/record/155453},
}