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| Hauptseite > Publikationsdatenbank > Magnetic correlations in HoxTb2-xTi2O7 > print |
| 001 | 15570 | ||
| 005 | 20250129094311.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevB.83.144413 |2 DOI |
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| 041 | _ | _ | |a eng |
| 082 | _ | _ | |a 530 |
| 084 | _ | _ | |2 WoS |a Physics, Condensed Matter |
| 100 | 1 | _ | |0 P:(DE-HGF)0 |a Chang, L. J. |b 0 |
| 245 | _ | _ | |a Magnetic correlations in HoxTb2-xTi2O7 |
| 260 | _ | _ | |a College Park, Md. |b APS |c 2011 |
| 300 | _ | _ | |a 144413 |
| 336 | 7 | _ | |a Journal Article |0 PUB:(DE-HGF)16 |2 PUB:(DE-HGF) |
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| 440 | _ | 0 | |0 4919 |a Physical Review B |v 83 |x 1098-0121 |y 14 |
| 500 | _ | _ | |a This work was supported in Taiwan by Grants No. NSC 96-2739-M-213-001, No. NSC 99-2112-M-007-020 (LJC), No. NSC 97-2628-M-002-011-MY3, and No. NTU 98R0066-65, -68 (Y.Z.C. and Y.J.K.). |
| 520 | _ | _ | |a Polycrystalline samples of HoxTb2-xTi2O7 (0 < x < 2) have been prepared and characterized for their structural and magnetic properties. The parent compounds of this solid solution are the spin ice Ho2Ti2O7 and the spin liquid Tb2Ti2O7. Specific-heat measurements on HoTbTi2O7 (x = 1.0) reveal the absence of a long-range order state above 0.5 K. The integrated entropies of all HoxTb2-xTi2O7 specimens up to 30 K scale well with the ratio of spin ice and spin liquid in the composition. The neutron diffraction spectrum of HoTbTi2O7 exhibits a dipolar spin-ice pattern and can be well described by mean-field theory for < 111 > Ising spins, nearest-neighbor exchange, and dipolar interactions. Inelastic neutron scattering on HoTbTi2O7 reveals two dispersionless excitations, one of similar to 2.5 meV out of the ground state, and a 4-meV transition out of an excited state. We argue that these data suggest that the very strong single-ion effects of Ho2Ti2O7 and Tb2Ti2O7 persist in the HoxTb2-xTi2O7(0 < x < 2) solid solution, whereas the Tb-Ho correlations are weak, resulting in small shifts in the energy scales but with no dramatic effect on the bulk properties. |
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