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@ARTICLE{Schweflinghaus:155845,
author = {Schweflinghaus, Benedikt and dos Santos Dias, Manuel and
Costa, Antonio T. and Lounis, Samir},
title = {{R}enormalization of electron self-energies via their
interaction with spin excitations: {A} first-principles
investigation},
journal = {Physical review / B},
volume = {89},
number = {23},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2014-04803},
pages = {235439},
year = {2014},
abstract = {Access to magnetic excitation spectra of single atoms
deposited on surfaces is nowadays possible by means of
low-temperature inelastic scanning tunneling spectroscopy.
We present a first-principles method for the calculation of
inelastic tunneling spectra utilizing the
Korringa-Kohn-Rostoker Green function method combined with
time-dependent density functional theory and many-body
perturbation theory. The key quantity is the electron
self-energy describing the coupling of the electrons to the
spin excitation within the adsorbate. By investigating Cr,
Mn, Fe, and Co adatoms on a Cu(111) substrate, we
spin-characterize the spectra and demonstrate that their
shapes are altered by the magnetization of the adatoms, of
the tip and the orbital decay into vacuum. Our method also
predicts spectral features more complex than the steps
obtained by simpler models for the adsorbate (e.g.,
localized spin models)},
cin = {PGI-1 / IAS-1},
ddc = {530},
cid = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)IAS-1-20090406},
pnm = {422 - Spin-based and quantum information (POF2-422)},
pid = {G:(DE-HGF)POF2-422},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000339049700008},
doi = {10.1103/PhysRevB.89.235439},
url = {https://juser.fz-juelich.de/record/155845},
}