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@ARTICLE{Rahmanizadeh:155920,
author = {Rahmanizadeh, K. and Wortmann, D. and Bihlmayer, G. and
Blügel, S.},
title = {{C}harge and orbital order at head-to-head domain walls in
{P}b{T}i{O}3},
journal = {Physical review / B},
volume = {90},
number = {11},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2014-04850},
pages = {115104},
year = {2014},
abstract = {At ferroelectric longitudinal domain walls there is an
uncompensated charge, which could form a two-dimensional
electron gas in the insulator. However, the uncompensated
charges can be accommodated by, e.g., defects or localized
states that split off from the conduction band. We carried
out density functional theory calculations to study these
scenarios in PbTiO3 with and without consideration of strong
correlation effects simulated via inclusion of a Hubbard
parameter U. The optimized structure and electronic
structure depend on the choice of this parameter: For
vanishing U, a broad, conducting domain wall is obtained,
while increasing U leads to localized Ti 3d states and an
insulating, sharp domain wall. We also investigated the
effects of varying the ferroelectric polarization on the
electronic structure of these domain walls.},
cin = {IAS-1 / PGI-1},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106},
pnm = {422 - Spin-based and quantum information (POF2-422)},
pid = {G:(DE-HGF)POF2-422},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000341239300004},
doi = {10.1103/PhysRevB.90.115104},
url = {https://juser.fz-juelich.de/record/155920},
}