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@PHDTHESIS{Kichin:155983,
author = {Kichin, Georgy},
title = {{S}ubmolecular imaging with single particleatomic force
sensors},
volume = {87},
school = {RWTH Aachen},
type = {Dr.},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {FZJ-2014-04903},
isbn = {978-3-89336-976-8},
series = {Schriften des Forschungszentrums Jülich. Reihe
Schlüsseltechnologien / Key Technologies},
pages = {140 S.},
year = {2014},
note = {RWTH Aachen, Diss., 2014},
abstract = {Scanning probe methods with decorated tips is a new trend
in surface study. An application of complex probe like a tip
with an attached single molecule or single atom allows to
get new details about the surface properties. It has been
shown that the scanning tunnelling hydrogen microscopy(STHM)
approach can reach atomic scale resolution and reveals
intermolecular interactions. Because of the complexity, this
new rapidly developing areais not yet fully understood. In
this work systematic studies of tips decorated with Xe,
H$_{2}$, D$_{2}$, CO, CH$_{4}$ was carried out. The tip with
a single atom or a single molecule creates asingle particle
sensor that simultaneously performs the function of an
atomic-scale force sensor and a signal transducer, which
couples the short-range force acting on the tip to the
tunnelling conductance of the junction. In some cases the
sensor-transducer function of the decorated STM tips can be
quantitatively calibrated. Differences in the performance of
the studied sensors suggest that the sensor functionality
can be modified by tuning the interaction between the sensor
particle and the STM tip. Based on force-field calculations,
theoretical analysis of the single particle sensor shows an
interrelation between the relative movement of the particle
on the tip and contrast structure of the surface images.},
keywords = {Dissertation (GND)},
cin = {PGI-3},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {899 - ohne Topic (POF3-899)},
pid = {G:(DE-HGF)POF3-899},
typ = {PUB:(DE-HGF)11},
url = {https://juser.fz-juelich.de/record/155983},
}