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@ARTICLE{Fukushima:155986,
author = {Fukushima, T. and Katayama-Yoshida, H. and Sato, K. and
Bihlmayer, G. and Mavropoulos, P. and Bauer, David and
Zeller, R. and Dederichs, P. H.},
title = {{H}ubbard {U} calculations for gap states in dilute
magnetic semiconductors},
journal = {Journal of physics / Condensed matter},
volume = {26},
number = {27},
issn = {1361-648X},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {FZJ-2014-04906},
pages = {274202},
year = {2014},
abstract = {On the basis of constrained density functional theory, we
present ab initio calculations for the Hubbard U parameter
of transition metal impurities in dilute magnetic
semiconductors, choosing Mn in GaN as an example. The
calculations are performed by two methods: (i) the
Korringa–Kohn–Rostoker (KKR) Green function method for a
single Mn impurity in GaN and (ii) the full-potential
linearized augmented plane-wave (FLAPW) method for a large
supercell of GaN with a single Mn impurity in each cell. By
changing the occupancy of the majority t2 gap state of Mn,
we determine the U parameter either from the total energy
differences E(N + 1) and E(N − 1) of the (N ± 1)-electron
excited states with respect to the ground state energy E(N),
or by using the single-particle energies for $n_0\pm \frac
{1}{2}$ occupancies around the charge-neutral occupancy n0
(Janak's transition state model). The two methods give
nearly identical results. Moreover the values calculated by
the supercell method agree quite well with the Green
function values. We point out an important difference
between the 'global' U parameter calculated using Janak's
theorem and the 'local' U of the Hubbard model.},
cin = {IAS-1 / PGI-1 / IAS-3 / PGI-2 / JARA-FIT / JARA-HPC},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
I:(DE-Juel1)IAS-3-20090406 / I:(DE-Juel1)PGI-2-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {422 - Spin-based and quantum information (POF2-422) /
Quantum description of nanoscale processes in materials
science $(jiff02_20120501)$},
pid = {G:(DE-HGF)POF2-422 / $G:(DE-Juel1)jiff02_20120501$},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000338702600005},
doi = {10.1088/0953-8984/26/27/274202},
url = {https://juser.fz-juelich.de/record/155986},
}