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000015731 084__ $$2WoS$$aPhysics, Condensed Matter
000015731 1001_ $$0P:(DE-HGF)0$$aGoremychkin, E.A.$$b0
000015731 245__ $$aSpatial inhomogeneity in RFeAsO(1-x)F(x) (R = Pr, Nd) determined from rare-earth crystal-field excitations
000015731 260__ $$aCollege Park, Md.$$bAPS$$c2011
000015731 300__ $$a212505
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000015731 440_0 $$04919$$aPhysical Review B$$v83$$x1098-0121
000015731 500__ $$aWe acknowledge useful discussions with E. Dagotto and assistance in the neutron-scattering experiments from O. Garlea (ORNL), T. Guidi (ISIS), A. Orecchini (ILL), and M. Koza (ILL). Research at Argonne and Oak Ridge is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division and Scientific User Facilities Division (Argonne Contract No. DE-AC02-06CH11357).
000015731 520__ $$aWe report inelastic neutron-scattering measurements of crystal-field transitions in PrFeAsO, PrFeAsO0.87F0.13, and NdFeAsO0.85F0.15. Doping with fluorine produces additional crystal-field excitations, providing evidence that there are two distinct charge environments around the rare-earth ions, with probabilities that are consistent with a random distribution of dopants on the oxygen sites. The 4f electrons of the Pr3+ and Nd3+ ions have nonmagnetic and magnetic ground states, respectively, indicating that the enhancement of T-c compared to LaFeAsO1-xFx is not due to rare-earth magnetism.
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000015731 7001_ $$0P:(DE-HGF)0$$aOsborn, R.$$b1
000015731 7001_ $$0P:(DE-HGF)0$$aWang, C.H.$$b2
000015731 7001_ $$0P:(DE-HGF)0$$aLumsden, M.D.$$b3
000015731 7001_ $$0P:(DE-HGF)0$$aMcGuire, M.A.$$b4
000015731 7001_ $$0P:(DE-HGF)0$$aSefat, A.S.$$b5
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