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@ARTICLE{Jablonowski:16336,
author = {Jablonowski, N.D. and Linden, A. and Köppchen, St. and
Thiele, B. and Hofmann, D. and Burauel, P.},
title = {{D}ry-wet cycles increase pesticide residue release from
soil},
journal = {Environmental toxicology and chemistry},
volume = {31},
issn = {0730-7268},
address = {Lawrence, KS},
publisher = {SETAC [u.a.]},
reportid = {PreJuSER-16336},
pages = {1941 - 1947},
year = {2012},
note = {We acknowledge with thanks the initial support and funding
of the lysimeter studies and the provision of the chemical
standards by Bayer Crop Science. The accurate and reliable
laboratory assistance and DOC/TN analyses by M. Krause are
highly appreciated. We also thank the technical staff of
IBG-3 for the continuous maintenance of the outdoor
lysimeters. The entire experiment was conducted at IBG-3:
Agrosphere Institute. Thanks to A. Wagner for his reliable
help with LaTeX.},
comment = {..},
booktitle = {..},
abstract = {Soil drying and rewetting may alter the release and
availability of aged pesticide residues in soils. A
laboratory experiment was conducted to evaluate the
influence of soil drying and wetting on the release of
pesticide residues. Soil containing environmentally
long-term aged (9-17 years) (14) C-labeled residues of the
herbicides ethidimuron (ETD) and methabenzthiazuron (MBT)
and the fungicide anilazine (ANI) showed a significantly
higher release of (14) C activity in water extracts of
previously dried soil compared to constantly moistened soil
throughout all samples (ETD: p < 0.1, MBT and ANI: p <
0.01). The extracted (14) C activity accounted for $44\%$
(ETD), $15\%$ (MBT), and $20\%$ (ANI) of total residual (14)
C activity in the samples after 20 successive dry-wet
cycles, in contrast to $15\%$ (ETD), $5\%$ (MBT), and $6\%$
(ANI) in extracts of constantly moistened soils. In the
dry-wet soils, the dissolved organic carbon (DOC) content
correlated with the measured (14) C activity in the aqueous
liquids and indicated a potential association of DOC with
the pesticide molecules. Liquid chromatography MS/MS
analyses of the water extracts of dry-wet soils revealed ETD
and MBT in detectable amounts, accounting for 1.83 and
$0.01\%,$ respectively, of total applied water-extractable
parent compound per soil layer. These findings demonstrate a
potential remobilization of environmentally aged pesticide
residue fractions from soils due to abiotic stresses such as
wet-dry cycles.},
keywords = {J (WoSType)},
cin = {IBG-2 / IBG-3 / ZCH},
ddc = {690},
cid = {I:(DE-Juel1)IBG-2-20101118 / I:(DE-Juel1)IBG-3-20101118 /
I:(DE-Juel1)ZCH-20090406},
pnm = {Terrestrische Umwelt},
pid = {G:(DE-Juel1)FUEK407},
shelfmark = {Environmental Sciences / Toxicology},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:22782855},
pmc = {pmc:PMC3465778},
UT = {WOS:000307938500004},
doi = {10.1002/etc.1851},
url = {https://juser.fz-juelich.de/record/16336},
}