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000016345 084__ $$2WoS$$aPhysics, Condensed Matter
000016345 1001_ $$0P:(DE-Juel1)VDB39593$$aFournier, N.$$b0$$uFZJ
000016345 245__ $$aForce-controlled lifting of molecular wires
000016345 260__ $$aCollege Park, Md.$$bAPS$$c2011
000016345 300__ $$a035435
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000016345 500__ $$3POF3_Assignment on 2016-02-29
000016345 500__ $$aWe gratefully acknowledge fruitful discussions with M. Rohlfing (Universitat Osnabruck) and C. Toher (TU Dresden), as well as the financial support from the Deutsche Forschungsgemeinschaft (DFG SPP 1243). R. T. acknowledges support by the Helmholtz-Gemeinschaft.
000016345 520__ $$aLifting a single molecular wire off the surface with a combined frequency-modulated atomic force and tunneling microscope it is possible to monitor the evolution of both the wire configuration and the contacts simultaneously with the transport conductance experiment. In particular, critical points where individual bonds to the surface are broken and instabilities where the wire is prone to change its contact configuration can be identified in the force gradient and dissipation responses of the junction. This additional mechanical information can be used to unambiguously determine the conductance of a true molecular wire, that is, of a molecule that is contacted via a pointlike "crocodile clip" to each of the electrodes but is otherwise free.
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000016345 7001_ $$0P:(DE-Juel1)VDB82898$$aWagner, C.$$b1$$uFZJ
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000016345 7001_ $$0P:(DE-Juel1)VDB73384$$aTemirov, R.$$b3$$uFZJ
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