TY  - JOUR
AU  - Fournier, N.
AU  - Wagner, C.
AU  - Weiss, C.
AU  - Temirov, R.
AU  - Tautz, F.S.
TI  - Force-controlled lifting of molecular wires
JO  - Physical review / B
VL  - 84
IS  - 3
SN  - 1098-0121
CY  - College Park, Md.
PB  - APS
M1  - PreJuSER-16345
SP  - 035435
PY  - 2011
N1  - We gratefully acknowledge fruitful discussions with M. Rohlfing (Universitat Osnabruck) and C. Toher (TU Dresden), as well as the financial support from the Deutsche Forschungsgemeinschaft (DFG SPP 1243). R. T. acknowledges support by the Helmholtz-Gemeinschaft.
AB  - Lifting a single molecular wire off the surface with a combined frequency-modulated atomic force and tunneling microscope it is possible to monitor the evolution of both the wire configuration and the contacts simultaneously with the transport conductance experiment. In particular, critical points where individual bonds to the surface are broken and instabilities where the wire is prone to change its contact configuration can be identified in the force gradient and dissipation responses of the junction. This additional mechanical information can be used to unambiguously determine the conductance of a true molecular wire, that is, of a molecule that is contacted via a pointlike "crocodile clip" to each of the electrodes but is otherwise free.
KW  - J (WoSType)
LB  - PUB:(DE-HGF)16
UR  - <Go to ISI:>//WOS:000293128900026
DO  - DOI:10.1103/PhysRevB.84.035435
UR  - https://juser.fz-juelich.de/record/16345
ER  -