Hauptseite > Publikationsdatenbank > Lattice dynamics in the FeSb3 skutterudite > print

001     16384
005     20250129094148.0
024 7 _ |a 10.1103/PhysRevB.84.064302
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037 _ _ |a PreJuSER-16384
041 _ _ |a eng
082 _ _ |a 530
084 _ _ |2 WoS
|a Physics, Condensed Matter
100 1 _ |0 P:(DE-Juel1)VDB73735
|a Möchel, A.
|b 0
|u FZJ
245 _ _ |a Lattice dynamics in the FeSb3 skutterudite
260 _ _ |a College Park, Md.
|b APS
|c 2011
300 _ _ |a 064302
336 7 _ |a Journal Article
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440 _ 0 |0 4919
|a Physical Review B
|v 84
|x 1098-0121
|y 6
500 _ _ |a We thank Dr. H.-C. Wille and D. Bessas for their support during the NIS measurements and Dr. J. C. Feldman for making his calculation data16 available. We thank Dr. B. C. Sales for providing the CoSb3 and EuFe4Sb12 samples.17 The European Synchrotron Radiation Facility and the Advanced Photon Source are acknowledged for provision of synchrotron radiation beam time at the nuclear resonance station ID18 and ID22N and the high-energy station 6-ID-D, respectively. R. H. acknowledges support from the Helmholtz University Young Investigator Group "Lattice Dynamics in Emerging Functional Materials". F. G. acknowledges the financial support of the Fonds National de la Recherche Scientifique, Belgium (Grants No. 9.456595 and No. 1.5.064.05). The research at the University of Oregon was funded by the National Science Foundation under Grant No. DMR 0907049 and supported in part by ONR Grant No. N00014-07-1-0358 and by the Army Research Laboratory under Agreement No. W911NF-07-2-0083.
520 _ _ |a Thin films of FeSb3 were characterized by electronic transport, magnetometry, x-ray diffraction, Fe-57 and Sb-121 nuclear inelastic scattering, and Fe-57 Mossbauer spectroscopy. Resistivity and magnetometry measurements reveal semiconducting behavior with a 16.3(4) meV band gap and an effective paramagnetic moment of 0.57(6) mu(B), respectively. A systematic comparison of the lattice dynamics with CoSb3 and EuFe4Sb12 reveals that the Fe4Sb12 framework is softer than the Co4Sb12 framework, and that the observed softening and the associated lowering of the lattice thermal conductivity in the RFe4Sb12 filled skutterudites are not only related to the filler but also to the Fe4Sb12 framework.
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