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@ARTICLE{Berns:16387,
author = {Berns, A.E. and Bubici, S. and De Pasquale, C. and Alonzo,
G. and Conte, P.},
title = {{A}pplicability of solid state fast field cycling {NMR}
relaxometry in understanding relaxation properties of leaves
and leaf-litters},
journal = {Organic geochemistry},
volume = {42},
issn = {0146-6380},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PreJuSER-16387},
pages = {978 - 984},
year = {2011},
note = {P.C. acknowledges Forschungszentrum Julich GmbH (Germany)
for having invited him as visiting scientist at the NMR
centre of the Institute of Bio- and Geosciences, IBG-3:
Agrosphere. FFC NMR measurements were done at the Universita
degli Studi di Palermo. This work was partially funded by
Ce.R.T.A. s.c.r.l. (Centri Regionali per le Tecnologie
Alimentari; http://www.certa.it/default.asp)},
abstract = {Inversion recovery high field solid state (SS) H-1 NMR
spectroscopy and fast field cycling (FFC) NMR relaxometry
have been applied on dried leaves and leaf-litters from a
reafforestated area in central Sicily (Italy) in order to
evaluate relaxation properties in both slow (1 <<
omega(2)(0)tau(2)(c)) and fast (1 >> omega(2)(0)tau(2)(c))
motion regimes. Namely, SS H-1 NMR spectroscopy (i.e. slow
motion regime conditions) revealed that two relaxation
components (a fast and a slow one) can be identified in all
the leaves and leaf-litter samples. The fast component was
assigned to small sized plant metabolites, whereas the slow
one was attributed to slowly tumbling macropolymeric
molecules. FFC NMR relaxometry (i.e. fast motion regime
conditions) indicated that intra-and inter-segmental
motional contributions to plant relaxation occur, depending
on the nature of the plant sample under investigation. The
present study represents the first example of a combination
of high and low resolution NMR techniques for the
understanding of the dynamics properties of environmentally
relevant soft matter such as leaves and leaf-litters. These
materials are considered among the main contributors for the
synthesis of natural organic matter. For this reason, a
comprehension of their basic molecular dynamics properties
is a crucial point to evaluate their effect on, e.g., carbon
cycle, fate of organic and inorganic pollutants, and
microbial biomass grow. (C) 2011 Elsevier Ltd. All rights
reserved.},
keywords = {J (WoSType)},
cin = {IBG-3},
ddc = {540},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {Terrestrische Umwelt},
pid = {G:(DE-Juel1)FUEK407},
shelfmark = {Geochemistry $\&$ Geophysics},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000295215300012},
doi = {10.1016/j.orggeochem.2011.04.006},
url = {https://juser.fz-juelich.de/record/16387},
}