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000016413 0247_ $$2DOI$$a10.1016/j.chemosphere.2011.03.057
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000016413 084__ $$2WoS$$aEnvironmental Sciences
000016413 1001_ $$0P:(DE-Juel1)VDB100854$$aLi, C.L.$$b0$$uFZJ
000016413 245__ $$aEffect of structural composition of humic acids on the sorption of a branched nonylphenol isomer
000016413 260__ $$aAmsterdam [u.a.]$$bElsevier Science$$c2011
000016413 300__ $$a409 - 414
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000016413 440_0 $$01228$$aChemosphere$$v84$$x0045-6535$$y4
000016413 500__ $$3POF3_Assignment on 2016-02-29
000016413 500__ $$aChengliang Li was supported by a scholarship from the Deutscher Akademischer Austausch Dienst (DAAD). This study was financed by the National Natural Science Foundation of China (Project Nos.: 20777033 and 20977043). We thank Mr. Jun Shan and Mr. Xuesen Bian for their kind help in sampling sediments from the Yangtze River.
000016413 520__ $$aBy using dialysis equilibrium experiments, the sorption of a branched nonylphenol isomer [4-(1-ethyl-1,3-dimethylpentyl)-phenol] (NP111) on various humic acids (HAs) isolated from river sediments and two reference HAs was studied. The HAs were characterized by solid-state (13)C direct polarization/magic angle spinning nuclear magnetic resonance ((13)C DP/MAS NMR) spectroscopy. Sorption isotherms of NP111 on HAs were described by a linear model. The organic carbon-normalized sorption coefficient (K(OC)) ranged from 2.3×10(3) to 1.5×10(4)Lkg(-1). Interestingly, a clear correlation between K(OC) value and alkyl C content was observed, indicating that the aliphaticity of HAs markedly dominates the sorption of NP111. These new mechanistic insights about the NP111 sorption indicate that the fate of nonylphenols in soil or sediment depends not only on the content of HA, but also on its structural composition.
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000016413 588__ $$aDataset connected to Web of Science, Pubmed
000016413 65320 $$2Author$$aBranched nonylphenol
000016413 65320 $$2Author$$aSorption
000016413 65320 $$2Author$$aHumic acids
000016413 65320 $$2Author$$aNMR
000016413 65320 $$2Author$$aAliphaticity
000016413 650_2 $$2MeSH$$aAdsorption
000016413 650_2 $$2MeSH$$aGeologic Sediments: chemistry
000016413 650_2 $$2MeSH$$aHumic Substances
000016413 650_2 $$2MeSH$$aIsomerism
000016413 650_2 $$2MeSH$$aLinear Models
000016413 650_2 $$2MeSH$$aMagnetic Resonance Spectroscopy
000016413 650_2 $$2MeSH$$aModels, Chemical
000016413 650_2 $$2MeSH$$aMolecular Structure
000016413 650_2 $$2MeSH$$aPhenols: chemistry
000016413 650_2 $$2MeSH$$aWater Pollutants, Chemical: chemistry
000016413 650_7 $$00$$2NLM Chemicals$$aHumic Substances
000016413 650_7 $$00$$2NLM Chemicals$$aPhenols
000016413 650_7 $$00$$2NLM Chemicals$$aWater Pollutants, Chemical
000016413 650_7 $$025154-52-3$$2NLM Chemicals$$anonylphenol
000016413 650_7 $$2WoSType$$aJ
000016413 7001_ $$0P:(DE-Juel1)129438$$aBerns, A.E.$$b1$$uFZJ
000016413 7001_ $$0P:(DE-HGF)0$$aSchaffer, A.$$b2
000016413 7001_ $$0P:(DE-Juel1)VDB100855$$aSequaris, J.M.$$b3$$uFZJ
000016413 7001_ $$0P:(DE-Juel1)129549$$aVereecken, H.$$b4$$uFZJ
000016413 7001_ $$0P:(DE-Juel1)VDB89513$$aJi, R.$$b5$$uFZJ
000016413 7001_ $$0P:(DE-Juel1)129484$$aKlumpp, E.$$b6$$uFZJ
000016413 773__ $$0PERI:(DE-600)1496851-4$$a10.1016/j.chemosphere.2011.03.057$$gVol. 84, p. 409 - 414$$p409 - 414$$q84<409 - 414$$tChemosphere$$v84$$x0045-6535$$y2011
000016413 8567_ $$uhttp://dx.doi.org/10.1016/j.chemosphere.2011.03.057
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