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@PHDTHESIS{Neucheva:16431,
key = {16431},
othercontributors = {Neucheva, Olga},
title = {{I}nvestigation of a metal-organic interface - realization
and understanding of a molecular switch},
volume = {17},
school = {RWTH Aachen},
type = {Dr. (FH)},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {PreJuSER-16431},
isbn = {978-3-89336-650-7},
series = {Schriften des Forschungszentrums Jülich.
Schlüsseltechnologien / Key Technologies},
pages = {134 S.},
year = {2010},
note = {Record converted from JUWEL: 18.07.2013; RWTH Aachen,
Diss., 2010},
abstract = {The field of molecular organic electronics is an emerging
and very dynamic area. The continued trend to
miniaturisation, combined with increasing complexity and
cost of production in conventional semiconductor
electronics, forces companies to turn their attention to
alternatives that promise the next levels of scale at
significantly lower cost. After consumer electronic devices
based on organic transistors, such as TVs and book readers,
have already been presented, molecular electronics is
expected to offer the next breakthrough in feature size.
Unfortunately, most of the organic/metal interfaces contain
intrinsic defects that break the homogeneity of the
interface properties. In this thesis, the electronic and
structural properties of such defects were examined in order
to understand the influence of the inhomogeneities on the
quality of the interface layer. However, the main focus of
this work was the investigation of the local properties of a
single molecule. Taking advantage of the Scanning Tunnelling
Microscope's (STM's) ability to act as a local probe, a
single molecular switch was realized and studied. Moreover,
in close collaboration with theory groups, the underlying
mechanism driving the switching process was identified and
described. Besides the investigation of the switching
process, the ability of the STM to build nanostructures of
different shapes from large organic molecules was shown.
Knowing the parameters for realization and control of the
switching process and for building the molecular corrals,
the results of this investigation enable the reconstruction
of the studied molecular ensemble and its deployment in
electric molecular circuits, constituting a next step
towards further miniaturization of electronic devices.},
cin = {PGI-3},
ddc = {500},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {Grundlagen für zukünftige Informationstechnologien},
pid = {G:(DE-Juel1)FUEK412},
typ = {PUB:(DE-HGF)11 / PUB:(DE-HGF)3},
url = {https://juser.fz-juelich.de/record/16431},
}