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@ARTICLE{Lennartz:16723,
author = {Lennartz, M.C. and Baumert, M. and Karthäuser, S. and
Albrecht, M. and Waser, R.},
title = {{D}ihydroxy (4-thiomorpholinomethyl) benzoic acids - {F}rom
molecular asymmetry to diode characteristics},
journal = {Langmuir},
volume = {27},
issn = {0743-7463},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {PreJuSER-16723},
year = {2011},
note = {This work was funded by the DFG (Grant SPP1243). We thank
P. Kowalzik for the preparation of the gold samples and A.
Besmehn for the execution of the XPS measurements.},
abstract = {One of the challenges in molecular electronics is to design
molecules which can be used as functional units in
electronic devices. The subject of our investigations is an
asymmetrical molecule,
dihydroxy(4-thiomorpholinomethyl)benzoic acid (TMBA), whose
structural and electronic properties are characterized. The
self-assembly behavior of TMBA on Au(111) surfaces resulting
in highly ordered monolayers is obtained using scanning
tunneling microscopy (STM). Furthermore, investigations on
the electronic properties of the combined metal/molecule
system reveal an orbital mediated tunneling process and
tunneling decay constants for the carboxylic and
thiomorpholino group. Thus, a diode-like character of TMBA
is shown to be caused by intrinsic electronic properties of
different molecular moieties.},
keywords = {J (WoSType)},
cin = {JARA-FIT / PGI-7},
ddc = {670},
cid = {$I:(DE-82)080009_20140620$ / I:(DE-Juel1)PGI-7-20110106},
pnm = {Grundlagen für zukünftige Informationstechnologien},
pid = {G:(DE-Juel1)FUEK412},
shelfmark = {Chemistry, Multidisciplinary / Chemistry, Physical /
Materials Science, Multidisciplinary},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:21749130},
UT = {WOS:000293662800082},
doi = {10.1021/la201206e},
url = {https://juser.fz-juelich.de/record/16723},
}