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@ARTICLE{Mensah:17086,
author = {Mensah, A.A. and Buchholz, A. and Mentel, T.F. and
Tillmann, R. and Kiendler-Scharr, A.},
title = {{A}erosol mass spectrometric measurements of stable crystal
hydrates of oxalates and inferred relative ionization
efficiency of water},
journal = {Journal of aerosol science},
volume = {42},
issn = {0021-8502},
address = {Amsterdam},
publisher = {Elsevier},
reportid = {PreJuSER-17086},
pages = {11 - 19},
year = {2011},
note = {Record converted from VDB: 12.11.2012},
abstract = {We investigated the crystal hydrates of ammonium oxalate,
potassium oxalate and oxalic acid as well as sodium oxalate.
By taking advantage of the different crystal water contents
we determined for the first time the relative ionization
efficiency of water (RIEH2O) in an Aerodyne Aerosol Mass
Spectrometer (AMS). The RIE is a key parameter for the
quantitative measurement of a compounds' aerosol particle
concentration with an AMS. Since the liquid water content of
an aerosol particle determines its physical and chemical
properties to a large extent, the knowledge of the water
content is of high scientific interest. The investigation of
the three salts led to a RIEH2O of 2. Application of this
RIEH2O and further analysis of oxalic acid revealed two
major characteristics, which need to be considered in future
when handling oxalic acid. First, oxalic acid aerosol
particles show a reduced crystal water content compared to
the thermodynamically stable and expected value when
produced under standard laboratory conditions. Second, solid
oxalic acid and its solutions show significant contamination
with ammonium when exposed to atmospheric air. These
findings were verified by high resolution mass spectrometry
and their implications for laboratory studies of hygroscopic
growth and CCN properties of oxalic acid are discussed. (C)
2010 Elsevier Ltd. All rights reserved.},
keywords = {J (WoSType)},
cin = {IEK-8},
ddc = {530},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK491},
shelfmark = {Engineering, Chemical / Environmental Sciences /
Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000286960200002},
doi = {10.1016/j.jaerosci.2010.10.003},
url = {https://juser.fz-juelich.de/record/17086},
}