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@ARTICLE{Hoffmann:1717,
author = {Hoffmann, L. and Kaufmann, M. and Spang, R. and Müller, R.
and Remedios, J. J. and Moore, D. P. and Volk, C. M. and von
Clarmann, T. and Riese, M.},
title = {{E}nvisat {MIPAS} measurements of {CFC}-11: retrieval,
validation, and climatology},
journal = {Atmospheric Chemistry and Physics},
volume = {8},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-1717},
pages = {3671 - 3688},
year = {2008},
note = {Record converted from VDB: 12.11.2012},
abstract = {From July 2002 to March 2004 the Michelson Interferometer
for Passive Atmospheric Sounding (MIPAS) aboard the European
Space Agency's Environmental Satellite (Envisat) measured
nearly continuously mid infrared limb radiance spectra.
These measurements are utilised to retrieve the global
distribution of the chlorofluorocarbon CFC-11 by applying a
new fast forward model for Envisat MIPAS and an accompanying
optimal estimation retrieval processor. A detailed analysis
shows that the total retrieval errors of the individual
CFC-11 volume mixing ratios are typically below $10\%$ in
the altitude range 10 to 25 km and that the systematic
components dominate. Contribution of a priori information to
the retrieval results are less than 5 to $10\%$ and the
vertical resolution of the observations is about 3 to 4 km
in the same vertical range. The data are successfully
validated by comparison with several other space
experiments, an airborne in-situ instrument, measurements
from ground-based networks, and independent Envisat MIPAS
analyses. The retrieval results from 425 000 Envisat MIPAS
limb scans are compiled to provide a new climatological data
set of CFC-11. The climatology shows significantly lower
CFC-11 abundances in the lower stratosphere compared with
the Reference Atmospheres for MIPAS (RAMstan V3.1)
climatology. Depending on the atmospheric conditions the
differences between the climatologies are up to 30 to 110
ppt (45 to $150\%)$ at 19 to 27 km altitude. Additionally,
time series of CFC-11 mean abundance and variability for
five latitudinal bands are presented. The observed CFC-11
distributions can be explained by the residual mean
circulation and large-scale eddy-tran sports in the upper
troposphere and lower stratosphere. The new CFC-11 data set
is well suited for further scientific studies.},
keywords = {J (WoSType)},
cin = {ICG-1 / JARA-SIM},
ddc = {550},
cid = {I:(DE-Juel1)VDB790 / I:(DE-Juel1)VDB1045},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000257516800018},
url = {https://juser.fz-juelich.de/record/1717},
}