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@ARTICLE{Taslimi:171705,
      author       = {Taslimi, Farzaneh and Gompper, Gerhard and Winkler, Roland
                      G.},
      title        = {{S}caffold {S}tructures by {T}elechelic {R}odlike
                      {P}olymers: {N}onequilibrium {S}tructural and {R}heological
                      {P}roperties under {S}hear {F}low},
      journal      = {Macromolecules},
      volume       = {47},
      number       = {19},
      issn         = {0024-9297},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2014-05274},
      pages        = {6946-6954},
      year         = {2014},
      abstract     = {The nonequilibrium structural and rheological properties of
                      suspension of rodlike polymers with attractive ends are
                      investigated by mesoscale hydrodynamic simulations. The
                      hybrid simulation approach combines the multiparticle
                      collision dynamics method for the fluid with molecular
                      dynamics simulations for the polymers. In equilibrium, the
                      rodlike polymers self-organize into scaffold-like network
                      structures above a critical density and attraction strength.
                      Shear flow induces significant structural changes. We
                      identify three major regimes. At low Weissenberg numbers,
                      the scaffold structure is compactified accompanied by a
                      phase separation into a fluid domain and a dense
                      scaffold-like structure. The shear viscosity shows a
                      Newtonian plateau, which is determined by the fluid layer.
                      At intermediated shear rates, shear bands appear with
                      bundles of polymers. Again, we observe a nearly Newtonian
                      viscosity regime governed by the fluid bands. At high shear
                      rates, any structure is dissolved and a paranematic phase
                      appears, with rods well aligned with the flow, and shear
                      thinning appears.},
      cin          = {IAS-2 / ICS-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IAS-2-20090406 / I:(DE-Juel1)ICS-2-20110106},
      pnm          = {451 - Soft Matter Composites (POF2-451)},
      pid          = {G:(DE-HGF)POF2-451},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000343196200046},
      doi          = {10.1021/ma501215t},
      url          = {https://juser.fz-juelich.de/record/171705},
}