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000172053 1001_ $$0P:(DE-HGF)0$$aNaboka, Michael$$b0
000172053 245__ $$aDirect Evidence of the Temperature-Induced Molecular Reorientation in Tetracene Thin Films on AlO$_{x}$ /Ni $_{3}$ Al(111)422
000172053 260__ $$aWashington, DC$$bSoc.$$c2014
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000172053 520__ $$aControl over the optical properties of the fluorescent organic layer plays a key role in the development of organic light-emitting diodes. A combination of near-edge X-ray absorption fine structure spectroscopy and X-ray photoelectron spectroscopy was used to study structural changes in thin films of tetracene on AlOx/Ni3Al(111). It is shown that upon deposition onto the cold (100 K) substrate, a monolayer of tetracene molecules adopts a disordered adsorption configuration with the molecular planes orientated almost parallel to the surface. Upon annealing at 280 K, the molecular packing changes and the tetracene units adopt a more upright orientation. The consequences of this orientational change for the luminescent properties of the molecular adlayer are discussed, in particular with regard to a quenching of the optical excitation by an electronic coupling of occupied and unoccupied molecular states to those of the metal substrate
000172053 536__ $$0G:(DE-HGF)POF2-422$$a422 - Spin-based and quantum information (POF2-422)$$cPOF2-422$$fPOF II$$x0
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000172053 7001_ $$0P:(DE-Juel1)128790$$aSubach, Sergey$$b1
000172053 7001_ $$0P:(DE-HGF)0$$aNefedov, Alexei$$b2
000172053 7001_ $$0P:(DE-Juel1)128791$$aTautz, Frank Stefan$$b3$$ufzj
000172053 7001_ $$0P:(DE-HGF)0$$aWöll, Christof$$b4$$eCorresponding Author
000172053 773__ $$0PERI:(DE-600)2256522-X$$a10.1021/jp507773f$$gVol. 118, no. 39, p. 22678 - 22682$$n39$$p22678 - 22682$$tThe @journal of physical chemistry <Washington, DC> / C$$v118$$x1932-7455$$y2014
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