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@ARTICLE{Naboka:172053,
      author       = {Naboka, Michael and Subach, Sergey and Nefedov, Alexei and
                      Tautz, Frank Stefan and Wöll, Christof},
      title        = {{D}irect {E}vidence of the {T}emperature-{I}nduced
                      {M}olecular {R}eorientation in {T}etracene {T}hin {F}ilms on
                      {A}l{O}$_{x}$ /{N}i $_{3}$ {A}l(111)422},
      journal      = {The journal of physical chemistry / C},
      volume       = {118},
      number       = {39},
      issn         = {1932-7455},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2014-05602},
      pages        = {22678 - 22682},
      year         = {2014},
      abstract     = {Control over the optical properties of the fluorescent
                      organic layer plays a key role in the development of organic
                      light-emitting diodes. A combination of near-edge X-ray
                      absorption fine structure spectroscopy and X-ray
                      photoelectron spectroscopy was used to study structural
                      changes in thin films of tetracene on AlOx/Ni3Al(111). It is
                      shown that upon deposition onto the cold (100 K) substrate,
                      a monolayer of tetracene molecules adopts a disordered
                      adsorption configuration with the molecular planes
                      orientated almost parallel to the surface. Upon annealing at
                      280 K, the molecular packing changes and the tetracene units
                      adopt a more upright orientation. The consequences of this
                      orientational change for the luminescent properties of the
                      molecular adlayer are discussed, in particular with regard
                      to a quenching of the optical excitation by an electronic
                      coupling of occupied and unoccupied molecular states to
                      those of the metal substrate},
      cin          = {PGI-3 / JARA-FIT},
      ddc          = {540},
      cid          = {I:(DE-Juel1)PGI-3-20110106 / $I:(DE-82)080009_20140620$},
      pnm          = {422 - Spin-based and quantum information (POF2-422)},
      pid          = {G:(DE-HGF)POF2-422},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000342652000031},
      doi          = {10.1021/jp507773f},
      url          = {https://juser.fz-juelich.de/record/172053},
}