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@ARTICLE{Kang:172146,
author = {Kang, Kyongok and Hong, J. S. and Dhont, Jan K.G.},
title = {{L}ocal {I}nterfacial {M}igration of {C}lay {P}articles
within an {O}il {D}roplet in an {A}queous {E}nvironment},
journal = {The journal of physical chemistry / C},
volume = {118},
number = {42},
issn = {1932-7455},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2014-05657},
pages = {24803 - 24810},
year = {2014},
abstract = {We discuss the interfacial migration due to Marangoni
forces of clay particles within an oil droplet that is
immersed in water, which is relevant for the formation
kinetics of Pickering emulsions. Hydrophilic (MMT) and
hydrophobic (OMT) clays are studied, where the hydrophilic
clay particles adsorb in the oil–water interface, contrary
to the hydrophobic clays. The feasibility of an
“image–time correlation technique” is discussed, in
order to probe the local interfacial migration velocities of
clay particles in the oil droplet. Here, correlation
functions are constructed from time-resolved images, in
order to quantify the local migration of clay particles.
Correlation functions are measured at different waiting
times, that is, the time after formation of the droplet. The
initial decay rate and the baseline of these correlation
functions depend on the waiting time in a qualitatively
different way for the two clays, which is attributed to the
different interfacial migration behavior for the
hydrophilic, adsorbing clays and the nonadsorbing,
hydrophobic clays as a result of the Marangoni effect.},
cin = {ICS-3},
ddc = {540},
cid = {I:(DE-Juel1)ICS-3-20110106},
pnm = {451 - Soft Matter Composites (POF2-451)},
pid = {G:(DE-HGF)POF2-451},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000343740300066},
doi = {10.1021/jp508333u},
url = {https://juser.fz-juelich.de/record/172146},
}