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@INPROCEEDINGS{Mehmood:172147,
author = {Mehmood, Khalid and Hofmann, Diana and Burauel, Peter and
Vereecken, Harry and Berns, Anne E.},
title = {{C}esium and strontium sorption behavior in amended
agricultural soils},
school = {Rheinische Friedrich-Wilhelms-Universität Bonn},
reportid = {FZJ-2014-05658},
year = {2014},
abstract = {Biogas digestates and biochar are emerging soil amendments.
Biochar is a byproduct of pyrolysis process which is thermal
decomposition of biomass to produce syngas and bio-oil. The
use of biochar for soil amendment is being promoted for
higher crop yields and carbon sequestration. Currently, the
numbers of biogas plants in Germany are increasing to meet
the new energy scenarios. The sustainability of biogas
industry requires proper disposal options for digestate.
Biogas digestates being rich in nutrients are beneficial to
enhance agricultural productions. Contrary to the
agronomical benefits of these organic amendments, their use
can influence the mobility and bioavailability of soil
contaminants due to nutrients competition and high organic
matter content. So far, the impact of such amendments on
highly problematic contaminants like radionuclides is not
truly accounted for.In the present study,
sorption-desorption behavior of cesium and strontium was
investigated in three soils of different origin and texture.
Two agricultural soils, a loamy sand and a silty soil, were
amended with biochar and digestate in separate experiments,
with field application rates of 25 Mg/ha and 34 Mg/ha,
respectively. For comparison a third soil, a forest soil,
was incubated without any amendment. The amendments were
mixed into the top 20 cm of the field soils, resulting in
final concentrations of 8-9 g biochar/Kg soil and 11-12 g
digestate/Kg soil. The soils were incubated for about six
months at room temperature. Sorption-desorption experiments
were performed with CsCl and SrCl2 after pre-equilibrating
the soils with CaCl2 solutions.The amendments with field
application rates did not have a significant effect on the
relevant soil parameters responsible for the sorption
behavior of the two radionuclides. Comparatively, the soil
type lead to distinctive differences in sorption-desorption
dynamics of the two radionuclides. Cesium showed a higher
affinity for silty soil followed by forest soil and lowest
for sandy soil. Comparatively, strontium displayed a lower
adsorption for all three soils, with a slightly higher
adsorption in silty soil and almost similar sorption for
both forest and sandy soils. We conclude that the applied
organic amendments with field application rates will not
deplete the FES (Frayed Edge Sites) responsible for cesium
sorption in mineral soils. Furthermore, with the present
application rates the increase in amount of organic matter
is not high enough to significantly affect the strontium
sorption in mineral soils. The desorption experiments showed
that about 1/3 of the adsorbed cesium was extractable in
silty soil and almost half was extractable in forest and
sandy soils. In case of strontium, about half was
extractable in the three soils. Similar to sorption, the
effect of amendments was negligible compared to the soil
type.},
month = {Apr},
date = {2014-04-27},
organization = {EGU General Assembly, Vienna
(Austria), 27 Apr 2014 - 2 May 2014},
subtyp = {After Call},
cin = {IBG-3},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {245 - Chemicals in the Environment (POF2-245) / 255 -
Terrestrial Systems: From Observation to Prediction
(POF3-255)},
pid = {G:(DE-HGF)POF2-245 / G:(DE-HGF)POF3-255},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/172147},
}