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@ARTICLE{Snijkers:172297,
      author       = {Snijkers, Frank and Cho, Hong Y. and Nese, Alper and
                      Matyjaszewski, Krzysztof and Pyckhout-Hintzen, Wim and
                      Vlassopoulos, Dimitris},
      title        = {{E}ffects of {C}ore {M}icrostructure on {S}tructure and
                      {D}ynamics of {S}tar {P}olymer {M}elts: {F}rom {P}olymeric
                      to {C}olloidal {R}esponse},
      journal      = {Macromolecules},
      volume       = {47},
      number       = {15},
      issn         = {1520-5835},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2014-05780},
      pages        = {5347 - 5356},
      year         = {2014},
      abstract     = {The structure and linear viscoelastic behavior of four
                      different model star polymer melts were investigated
                      experimentally. The star polymers were prepared via
                      different synthetic routes based on atom transfer radical
                      polymerization (ATRP). Stars with small elongated (linear
                      backbone) cores exhibited slight differences in the
                      asymmetry of the core, which however did not affect the
                      rheological properties significantly. The relaxation
                      behavior of these stars with an asymmetric core was
                      well-described by available tube models. On the other hand,
                      stars with large cross-linked cores exhibited a core–shell
                      morphology and their stress relaxation was dominated by a
                      power-law decay over about 8 decades, akin to gel-like soft
                      systems. This behavior reflected their liquid-like ordering
                      and small intercore distances, and bares analogueies to that
                      of interpenetrating soft colloids and microgels.},
      cin          = {ICS-1 / Neutronenstreuung ; JCNS-1 / JCNS (München) ;
                      Jülich Centre for Neutron Science JCNS (München) ;
                      JCNS-FRM-II},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106 /
                      I:(DE-Juel1)JCNS-FRM-II-20110218},
      pnm          = {451 - Soft Matter Composites (POF2-451) / 54G - JCNS
                      (POF2-54G24)},
      pid          = {G:(DE-HGF)POF2-451 / G:(DE-HGF)POF2-54G24},
      experiment   = {EXP:(DE-MLZ)KWS1-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000340350400055},
      doi          = {10.1021/ma5008336},
      url          = {https://juser.fz-juelich.de/record/172297},
}