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@ARTICLE{Sols:172397,
author = {Solís, Cecilia and Somacescu, Simona and Palafox, Elena
and Balaguer, María and Serra, José M.},
title = {{P}articular {T}ransport {P}roperties of {N}i{F}e 2 {O} 4
{T}hin {F}ilms at {H}igh {T}emperatures},
journal = {The journal of physical chemistry / C},
volume = {118},
number = {42},
issn = {1932-7447},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2014-05877},
pages = {24266 - 24273},
year = {2014},
abstract = {NiFe2O4 (NFO) thin films were deposited on quartz
substrates by rf magnetron sputtering, and the influence of
the deposition conditions on their physic-chemical
properties was studied. The films structure and the high
temperature transport properties were analyzed as a function
of the deposition temperature. The analysis of the total
conductivity up to 800 °C in different pO2 containing
atmospheres showed a distinct electronic behavior of the
films with regard to the bulk NFO material. Indeed, the thin
films exhibit p-type electronic conductivity, while the bulk
material is known to be a prevailing n-type electronic
conductor. This difference is ascribed to the dissimilar
concentration of Ni3+ in the thin films, as revealed by XPS
analysis at room temperature. The bulk material with a low
concentration of Ni3+ (Ni3+/Ni2+ ratio of 0.20) shows the
expected n-type electronic conduction via electron hopping
between Fe3+–Fe2+. On the other hand, the NFO thin films
annealed at 800 °C exhibit a Ni3+/Ni2+ ratio of 0.42 and
show p-type conduction via hole hopping between
Ni3+–Ni2+.},
cin = {IEK-1},
ddc = {540},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {122 - Power Plants (POF2-122)},
pid = {G:(DE-HGF)POF2-122},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000343740300008},
doi = {10.1021/jp506938k},
url = {https://juser.fz-juelich.de/record/172397},
}