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@ARTICLE{Autieri:172587,
author = {Autieri, C. and Koch, Erik and Pavarini, Eva},
title = {{M}echanism of structural phase transitions in
{KC}r{F}$_{3}$},
journal = {Physical review / B},
volume = {89},
number = {15},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2014-06050},
pages = {155109},
year = {2014},
abstract = {We study the origin of the cubic to tetragonal and
tetragonal to monoclinic structural transitions in KCrF3,
and the associated change in orbital order, paying
particular attention to the relevance of super-exchange in
both phases. We show that super-exchange is not the main
mechanism driving these transitions. Specifically, it is not
strong enough to be responsible for the high-temperature
cubic to tetragonal transition and does not yield the type
of orbital order observed in the monoclinic phase. The
energy difference between the tetragonal and the monoclinic
structure is tiny, and most likely results from the
interplay between volume, covalency, and localization
effects. The transition is rather driven by Slater exchange
than super-exchange. Nevertheless, once the monoclinic
distortions are present, super-exchange helps in stabilizing
the low-symmetry structure. The orbital order we obtain for
this monoclinic phase is consistent with the magnetic
transition at 80 K.},
cin = {IAS-3},
ddc = {530},
cid = {I:(DE-Juel1)IAS-3-20090406},
pnm = {422 - Spin-based and quantum information (POF2-422)},
pid = {G:(DE-HGF)POF2-422},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000334117500002},
doi = {10.1103/PhysRevB.89.155109},
url = {https://juser.fz-juelich.de/record/172587},
}