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000172802 1001_ $$0P:(DE-Juel1)142224$$aBabajani, Ninet$$b0$$eCorresponding Author$$ufzj
000172802 245__ $$aDirected Immobilization of Janus-AuNP in Heterometallic Nanogaps: a Key Step Toward Integration of Functional Molecular Units in Nanoelectronics
000172802 260__ $$aWashington, DC$$bSoc.$$c2014
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000172802 520__ $$aForming reliable and reproducible molecule−nanoelectrodecontacts is one of the key issues for the implementation of nanoparticles asfunctional units into nanoscale devices. Utilizing heterometallic electrodes andJanus-type nanoparticles equipped with molecules allowing selective bindingto a distinct electrode material represents a promising approach to achievethis goal. Here, the directed immobilization of individual Janus-type goldnanoparticles (AuNP) between heterometallic electrodes leading to theformation of asymmetric contacts in a highly controllable way is presented.The Janus-AuNP are stabilized by two types of ligands with different terminalgroups on opposite hemispheres. The heterometallic nanoelectrode gaps areformed by electron beam lithography in combination with a self-alignmentprocedure and are adjusted to the size of the Janus-AuNP. Thus, by choosingadequate molecular end group/metal combinations, the immobilizationdirection of the Janus-AuNP is highly controllable. These results demonstratethe striking potential of this approach for the building-up of novel nanoscale organic/inorganic hybrid architectures.
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000172802 7001_ $$0P:(DE-HGF)0$$aKaulen, Corinna$$b1
000172802 7001_ $$0P:(DE-HGF)0$$aHomberger, Melanie$$b2
000172802 7001_ $$0P:(DE-Juel1)136859$$aMennicken, Max$$b3$$ufzj
000172802 7001_ $$0P:(DE-HGF)0$$aWaser, Rainer$$b4
000172802 7001_ $$0P:(DE-HGF)0$$aSimon, Ulrich$$b5
000172802 7001_ $$0P:(DE-Juel1)130751$$aKarthäuser, Silvia$$b6$$ufzj
000172802 773__ $$0PERI:(DE-600)2256522-X$$a10.1021/jp5085179$$gVol. 118, no. 46, p. 27142 - 27149$$n46$$p27142 - 27149$$tThe @journal of physical chemistry <Washington, DC> / C$$v118$$x1932-7455$$y2014
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