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000172822 005__ 20210129214518.0
000172822 0247_ $$2doi$$a10.1103/PhysRevLett.113.226101
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000172822 1001_ $$0P:(DE-HGF)0$$aHapalpa, Prokop$$b0$$eCorresponding Author
000172822 245__ $$aOrigin of High-Resolution IETS-STM Images of Organic Molecules with Functionalized Tips
000172822 260__ $$aCollege Park, Md.$$bAPS$$c2014
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000172822 520__ $$aRecently, the family of high-resolution scanning probe imaging techniques using decorated tips has been complemented by a method based on inelastic electron tunneling spectroscopy (IETS). The new technique resolves the inner structure of organic molecules by mapping the vibrational energy of a single carbon monoxide (CO) molecule positioned at the apex of a scanning tunneling microscope (STM) tip. Here, we explain high-resolution IETS imaging by extending a model developed earlier for STM and atomic force microscopy (AFM) imaging with decorated tips. In particular, we show that the tip decorated with CO acts as a nanoscale sensor that changes the energy of its frustrated translation mode in response to changes of the local curvature of the surface potential. In addition, we show that high resolution AFM, STM, and IETS-STM images can deliver information about the charge distribution within molecules deposited on a surface. To demonstrate this, we extend our mechanical model by taking into account electrostatic forces acting on the decorated tip in the surface Hartree potential.
000172822 536__ $$0G:(DE-HGF)POF2-422$$a422 - Spin-based and quantum information (POF2-422)$$cPOF2-422$$fPOF II$$x0
000172822 7001_ $$0P:(DE-Juel1)128792$$aTemirov, Ruslan$$b1$$ufzj
000172822 7001_ $$0P:(DE-Juel1)128791$$aTautz, Frank Stefan$$b2$$ufzj
000172822 7001_ $$0P:(DE-HGF)0$$aJelinek, Pavel$$b3
000172822 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.113.226101$$n14$$p226101$$tPhysical review letters$$v113$$x0031-9007$$y2014
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