000172889 001__ 172889 000172889 005__ 20250129094220.0 000172889 0247_ $$2doi$$a10.1016/j.jpcs.2014.11.011 000172889 0247_ $$2ISSN$$a0022-3697 000172889 0247_ $$2ISSN$$a0369-8726 000172889 0247_ $$2ISSN$$a1879-2553 000172889 0247_ $$2WOS$$aWOS:000349505000005 000172889 0247_ $$2altmetric$$aaltmetric:21824397 000172889 037__ $$aFZJ-2014-06320 000172889 082__ $$a530 000172889 1001_ $$0P:(DE-Juel1)144500$$aKlobes, B.$$b0$$eCorresponding Author 000172889 245__ $$aHyperfine interactions in and lattice parameters of pyrochlore and defect fluorite ${\left({\mathrm{Eu}}_{1-x}{\mathrm{Nd}}_{x}\right)}_{2}{\mathrm{Zr}}_{m2}{\mathrm{O}}_{7}$ 000172889 260__ $$aNew York, NY [u.a.]$$bElsevier$$c2015 000172889 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1429109525_26846 000172889 3367_ $$2DataCite$$aOutput Types/Journal article 000172889 3367_ $$00$$2EndNote$$aJournal Article 000172889 3367_ $$2BibTeX$$aARTICLE 000172889 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000172889 3367_ $$2DRIVER$$aarticle 000172889 520__ $$aPyrochlore and defect fluorite (Eu1−xNdx)2Zr2O7 compounds (x = 0, 0.5 and 0.75) synthesized by a wet chemicalapproach were investigated using temperature dependent high energy X-ray diffraction as well as 151Eu Mössbauerspectroscopy. Diffraction data reveals an increase in lattice parameter with increasing Nd content, an increase thatis disproportionally large between x = 0.5 and 0.75. The 151Eu Mössbauer spectral parameters, i.e. isomer shift andquadrupole splitting, fall in separate regions for pyrochlore and defect fluorite type compounds. Between 80 - 350 K,the impact of the order-disorder, i.e. pyrochlore to defect fluorite, transition on isomer shift and quadrupole splittingis found to exceed the one due to lattice expansion. 000172889 536__ $$0G:(DE-HGF)POF3-161$$a161 - Nuclear Waste Management (POF3-161)$$cPOF3-161$$fPOF III$$x0 000172889 588__ $$aDataset connected to CrossRef, juser.fz-juelich.de 000172889 7001_ $$0P:(DE-Juel1)142526$$aFinkeldei, S.$$b1 000172889 7001_ $$0P:(DE-Juel1)157665$$aRöhrig, Wilbert$$b2 000172889 7001_ $$0P:(DE-Juel1)130324$$aBosbach, D.$$b3 000172889 7001_ $$0P:(DE-HGF)0$$aHermann, R. P.$$b4 000172889 773__ $$0PERI:(DE-600)1491914-x$$a10.1016/j.jpcs.2014.11.011$$gp. S0022369714002844$$p43–48$$tJournal of physics and chemistry of solids$$v79$$x0022-3697$$y2015 000172889 8564_ $$uhttps://juser.fz-juelich.de/record/172889/files/FZJ-2014-06320.pdf$$yRestricted 000172889 909CO $$ooai:juser.fz-juelich.de:172889$$pVDB 000172889 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR 000172889 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index 000172889 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded 000172889 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection 000172889 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List 000172889 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS 000172889 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline 000172889 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz 000172889 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences 000172889 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF < 5 000172889 9141_ $$y2015 000172889 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)144500$$aForschungszentrum Jülich GmbH$$b0$$kFZJ 000172889 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)142526$$aForschungszentrum Jülich GmbH$$b1$$kFZJ 000172889 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130324$$aForschungszentrum Jülich GmbH$$b3$$kFZJ 000172889 9130_ $$0G:(DE-HGF)POF2-142$$1G:(DE-HGF)POF2-140$$2G:(DE-HGF)POF2-100$$aDE-HGF$$bEnergie$$lNukleare Sicherheitsforschung$$vSafety Research for Nuclear Waste Disposal$$x0 000172889 9131_ $$0G:(DE-HGF)POF3-161$$1G:(DE-HGF)POF3-160$$2G:(DE-HGF)POF3-100$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bEnergie$$lNukleare Entsorgung und Sicherheit sowie Strahlenforschung$$vNuclear Waste Management$$x0 000172889 9201_ $$0I:(DE-Juel1)IEK-6-20101013$$kIEK-6$$lNukleare Entsorgung und Reaktorsicherheit$$x0 000172889 9201_ $$0I:(DE-Juel1)JCNS-2-20110106$$kJCNS-2$$lStreumethoden$$x1 000172889 9201_ $$0I:(DE-82)080009_20140620$$kJARA-FIT$$lJARA-FIT$$x2 000172889 9201_ $$0I:(DE-Juel1)PGI-4-20110106$$kPGI-4$$lStreumethoden$$x3 000172889 980__ $$ajournal 000172889 980__ $$aVDB 000172889 980__ $$aI:(DE-Juel1)IEK-6-20101013 000172889 980__ $$aI:(DE-Juel1)JCNS-2-20110106 000172889 980__ $$aI:(DE-82)080009_20140620 000172889 980__ $$aI:(DE-Juel1)PGI-4-20110106 000172889 980__ $$aUNRESTRICTED 000172889 981__ $$aI:(DE-Juel1)IFN-2-20101013 000172889 981__ $$aI:(DE-Juel1)JCNS-2-20110106 000172889 981__ $$aI:(DE-Juel1)JCNS-2-20110106 000172889 981__ $$aI:(DE-Juel1)PGI-4-20110106