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@ARTICLE{Chang:173060,
      author       = {Chang, Shery L. Y. and Singh, Archana and Hocking, Rosalie
                      K. and Dwyer, Christian and Spiccia, Leone},
      title        = {{N}anoscale structural disorder in manganese oxide
                      particles embedded in {N}afion},
      journal      = {Journal of materials chemistry / A},
      volume       = {2},
      issn         = {2050-7488},
      address      = {London {[u.a.]},
      publisher    = {RSC},
      reportid     = {FZJ-2014-06473},
      pages        = {3730 - 3733},
      year         = {2014},
      abstract     = {Earlier studies have shown that manganese oxide particles
                      derived from a manganese molecular complex embedded in a
                      Nafion film have one order of magnitude higher
                      water-oxidation catalytic activity per manganese compared to
                      many unsupported solid-state manganese oxide particles.
                      Using transmission electron microscopy and electron
                      scattering simulations, we have shown that the
                      sodium-birnessite phase particles in Nafion exhibit an
                      exceptionally high degree of layer mis-registration, and a
                      high concentration of Mn vacancies, compared to the
                      synthetic birnessite nanoparticles. It is therefore proposed
                      that the differences in the activities correlate with the
                      degree of disorder in the manganese oxide particles.},
      cin          = {PGI-5},
      ddc          = {540},
      cid          = {I:(DE-Juel1)PGI-5-20110106},
      pnm          = {424 - Exploratory materials and phenomena (POF2-424) / 42G
                      - Peter Grünberg-Centre (PG-C) (POF2-42G41)},
      pid          = {G:(DE-HGF)POF2-424 / G:(DE-HGF)POF2-42G41},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000331893700006},
      doi          = {10.1039/c3ta14738j},
      url          = {https://juser.fz-juelich.de/record/173060},
}