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@ARTICLE{Rosn:173280,
author = {Rosén, E. and Schweika, W. and Meven, M. and Leo, N. R.
and Meier, D. and Fiebig, M. and Kuo, C.-Y. and Pi, T.-W.
and Hu, Z. and Valldor, M. and Reim, Johannes and Schmidt,
M.},
title = {{S}tructural invariance upon antiferromagnetic ordering in
geometrically frustrated swedenborgite, {C}a{B}a{C}o 2 {F}e
2 {O} 7},
journal = {Journal of applied crystallography},
volume = {47},
number = {6},
issn = {1600-5767},
address = {Copenhagen},
publisher = {Munksgaard},
reportid = {FZJ-2014-06691},
pages = {2038 - 2047},
year = {2014},
abstract = {Centimetre-sized single crystals of high-quality
CaBaCo2Fe2O7 were synthesized by the optical floating zone
technique. The metal-to-metal stoichiometry and oxygen
content were confirmed by spectroscopy and thermal reduction
experiments. The hexagonal symmetry P63mc (No. 186) well
describes the powder X-ray and neutron diffraction as well
as single-crystal neutron diffraction at all measured
temperatures. This symmetry is also consistent with optical
second harmonic generation data obtained between 10 and 295
K. However, a satisfactory structure description from
single-crystal neutron diffraction data needs an oxygen
split position. Specific heat, magnetic susceptibility and
powder neutron diffraction data indicate a magnetic phase
transition at TN = 159 K to an antiferromagnetic ground
state, but with a persisting hexagonal symmetry and
intrinsic geometric frustration.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS (München) ; Jülich
Centre for Neutron Science JCNS (München) ; JCNS-FRM-II},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {422 - Spin-based and quantum information (POF2-422) / 424 -
Exploratory materials and phenomena (POF2-424) / 542 -
Neutrons (POF2-542) / 544 - In-house Research with PNI
(POF2-544) / 54G - JCNS (POF2-54G24)},
pid = {G:(DE-HGF)POF2-422 / G:(DE-HGF)POF2-424 /
G:(DE-HGF)POF2-542 / G:(DE-HGF)POF2-544 /
G:(DE-HGF)POF2-54G24},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000345877900027},
doi = {10.1107/S1600576714023528},
url = {https://juser.fz-juelich.de/record/173280},
}