Hauptseite > Publikationsdatenbank > Electronic structure trends in the Sr(n+1)Ru(n)O(3n+1) family (n=1,2,3) > print |
001 | 17644 | ||
005 | 20240625095033.0 | ||
024 | 7 | _ | |a 10.1103/PhysRevB.83.165121 |2 DOI |
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041 | _ | _ | |a eng |
082 | _ | _ | |a 530 |
084 | _ | _ | |2 WoS |a Physics, Condensed Matter |
100 | 1 | _ | |0 P:(DE-HGF)0 |a Malvestuto, M. |b 0 |
245 | _ | _ | |a Electronic structure trends in the Sr(n+1)Ru(n)O(3n+1) family (n=1,2,3) |
260 | _ | _ | |a College Park, Md. |b APS |c 2011 |
300 | _ | _ | |a 165121 |
336 | 7 | _ | |a Journal Article |0 PUB:(DE-HGF)16 |2 PUB:(DE-HGF) |
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440 | _ | 0 | |0 4919 |a Physical Review B |v 83 |x 1098-0121 |y 16 |
500 | _ | _ | |3 POF3_Assignment on 2016-02-29 |
500 | _ | _ | |a E.G. and E.P. acknowledge the Julich BlueGene/P Grant No. JIFF41, as well as financial support by the Deutsche Forschungsgemeinschaft through the research unit FOR 1346. |
520 | _ | _ | |a The identification of electronic states and the analysis of their evolution with n is key to understanding n-layered ruthenates. To this end, we combine polarization-dependent O 1s x-ray absorption spectroscopy, high-purity Srn+1RunO3n+1 (n = 1,2,3) single crystals, and ab initio and many-body calculations. We find that the energy splitting between the empty x(2) - y(2) and 3z(2) - 1 state is considerably smaller than previously suggested and that, remarkably, Sr bands are essential to understanding the spectra. At low energy, we identify the main difference among the materials with a substantial rearrangement of t(2g) orbital occupations with increasing n. This rearrangement is controlled by the interplay of Coulomb repulsion, dimensionality, and changes in the t(2g) crystal field. |
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856 | 7 | _ | |u http://dx.doi.org/10.1103/PhysRevB.83.165121 |
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