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000017658 0247_ $$2DOI$$a10.1016/j.susc.2011.02.024
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000017658 084__ $$2WoS$$aChemistry, Physical
000017658 084__ $$2WoS$$aPhysics, Condensed Matter
000017658 1001_ $$0P:(DE-HGF)0$$aKakudate, T.$$b0
000017658 245__ $$aInitial stage of adsorption of octithiophene molecules on Cu(111)
000017658 260__ $$aAmsterdam$$bElsevier$$c2011
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000017658 500__ $$3POF3_Assignment on 2016-02-29
000017658 500__ $$aThis work was supported in part by the World Premier International Research Center (WPI) Initiative on Materials Nanoarchitectonics, MEXT, Japan. T. N acknowledges the support of Grant-in-Aid for Scientific Research (A) (No. 22241030-2).
000017658 520__ $$aThe initial stage of the adsorption of octithiophene (8T) molecules on a Cu(111) surface is investigated using a scanning tunneling microscope at room temperature. We find a characteristic molecular chain structure of 8T molecules on a terrace of the Cu(111) surface, which has not been reported so far for adsorption of oligothiophene molecules on metal surfaces. Up to the adsorption of 0.26 monolayer (ML), 81 molecules in the molecular chain align with their long axis parallel to the Cu < 11-2 > direction. With increasing coverage, there appear 8T molecules that align with their long axis parallel to the Cu < 110 > direction. The appearance of different molecular orientations is understood by the decrease of the number of the adsorption sites for extending the molecular chains. Fragments of 8T molecules, such as single thiophene molecules, are also observed in this work. They are trapped only at the step edges of the Cu(111) surface at the beginning and later trapped in a small Cu(111) region surrounded by 8T molecules. (C) 2011 Elsevier B.V. All rights reserved.
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000017658 65320 $$2Author$$aOligothiophene
000017658 65320 $$2Author$$aOctithiophene
000017658 65320 $$2Author$$aAdsorption
000017658 65320 $$2Author$$aMolecular chain
000017658 65320 $$2Author$$aCu(111)
000017658 65320 $$2Author$$aScanning tunneling microscopy
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000017658 7001_ $$0P:(DE-Juel1)VDB87430$$aTsukamoto, S.$$b1$$uFZJ
000017658 7001_ $$0P:(DE-HGF)0$$aNakaya, M.$$b2
000017658 7001_ $$0P:(DE-HGF)0$$aNakayama, T.$$b3
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