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@ARTICLE{Kisner:17994,
author = {Kisner, A. and Stockmann, R. and Jansen, M. and Yegin, U.
and Offenhäusser, A. and Kubota, L. T. and Mourzina, Y.},
title = {{S}ensing small neurotransmitter enzyme interaction with
nanoporous gated ion-sensitive field effect transistors},
journal = {Biosensors and bioelectronics},
volume = {31},
number = {1},
issn = {0956-5663},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PreJuSER-17994},
pages = {157–163},
year = {2012},
note = {Record converted from VDB: 12.11.2012},
abstract = {Ion-sensitive field effect transistors with gates having a
high density of nanopores were fabricated and employed to
sense the neurotransmitter dopamine with high selectivity
and detectability at micromolar range. The nanoporous
structure of the gates was produced by applying a relatively
simple anodizing process, which yielded a porous alumina
layer with pores exhibiting a mean diameter ranging from 20
to 35 nm. Gate-source voltages of the transistors
demonstrated a pH-dependence that was linear over a wide
range and could be understood as changes in surface charges
during protonation and deprotonation. The large surface area
provided by the pores allowed the physical immobilization of
tyrosinase, which is an enzyme that oxidizes dopamine, on
the gates of the transistors, and thus, changes the
acid-base behavior on their surfaces.
Concentration-dependent dopamine interacting with
immobilized tyrosinase showed a linear dependence into a
physiological range of interest for dopamine concentration
in the changes of gate-source voltages. In comparison with
previous approaches, a response time relatively fast for
detecting dopamine was obtained. Additionally, selectivity
assays for other neurotransmitters that are abundantly found
in the brain were examined. These results demonstrate that
the nanoporous structure of ion-sensitive field effect
transistors can easily be used to immobilize specific enzyme
that can readily and selectively detect small
neurotransmitter molecule based on its acid-base interaction
with the receptor. Therefore, it could serve as a technology
platform for molecular studies of neurotransmitter-enzyme
binding and drugs screening.},
keywords = {Biosensing Techniques: instrumentation / Conductometry:
instrumentation / Electrodes / Enzymes, Immobilized:
chemistry / Equipment Design / Equipment Failure Analysis /
Ions / Monophenol Monooxygenase: chemistry / Nanostructures:
chemistry / Nanostructures: ultrastructure / Nanotechnology:
instrumentation / Neurotransmitter Agents: chemistry /
Porosity / Protein Binding / Protein Interaction Mapping:
instrumentation / Reproducibility of Results / Sensitivity
and Specificity / Transistors, Electronic / Enzymes,
Immobilized (NLM Chemicals) / Ions (NLM Chemicals) /
Neurotransmitter Agents (NLM Chemicals) / Monophenol
Monooxygenase (NLM Chemicals)},
cin = {ICS-8 / JARA-FIT / PGI-8},
ddc = {570},
cid = {I:(DE-Juel1)ICS-8-20110106 / $I:(DE-82)080009_20140620$ /
I:(DE-Juel1)PGI-8-20110106},
pnm = {Grundlagen für zukünftige Informationstechnologien /
BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung},
pid = {G:(DE-Juel1)FUEK412 / G:(DE-Juel1)FUEK505},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:22040747},
UT = {WOS:000300468400025},
doi = {10.1016/j.bios.2011.10.010},
url = {https://juser.fz-juelich.de/record/17994},
}