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000018271 084__ $$2WoS$$aChemistry, Physical
000018271 084__ $$2WoS$$aPhysics, Atomic, Molecular & Chemical
000018271 1001_ $$0P:(DE-HGF)0$$aLee, D.-K.$$b0
000018271 245__ $$aAn EMF cell with a nitrogen solid electrolyte - on the transference of nitrogen ions in yttria-stabilized zirconia
000018271 260__ $$aCambridge$$bRSC Publ.$$c2011
000018271 300__ $$a1239 - 1242
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000018271 440_0 $$04916$$aPhysical Chemistry Chemical Physics$$v13$$x1463-9076$$y3
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000018271 500__ $$aThis study (DFG Ja648/ 8-3, Le781/ 10-4) was funded by the German Science Foundation (DFG) within the priority program 1136 Substitution Effects in Ionic Solids.
000018271 520__ $$aThe mobility and electrochemical activity of nitrogen inside and/or at the surface of ionic compounds is of fundamental, as well as of possibly practical, relevance. In order to better understand the role of nitrogen anions in solid electrolytes, we measured the transference number of nitrogen in yttria-stabilized zirconia (YSZ) by a concentration cell technique as a function of oxygen activity at different temperatures in the range of 1023 ≤T/K≤ 1123. YSZ doped with 1.9 wt% of N (YSZ:N) turned out to have an appreciable nitrogen transference number, which increased from 0 to 0.1 with decreasing oxygen activity in the range of -20 < log a(O(2)) < -14. The stability of N in YSZ:N, however, has yet to be elucidated under oxidizing conditions.
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000018271 7001_ $$0P:(DE-HGF)0$$aFischer, C.C.$$b1
000018271 7001_ $$0P:(DE-Juel1)VDB85752$$aValov, I.$$b2$$uFZJ
000018271 7001_ $$0P:(DE-HGF)0$$aReinacher, J.$$b3
000018271 7001_ $$0P:(DE-HGF)0$$aStork, A.$$b4
000018271 7001_ $$0P:(DE-HGF)0$$aLerch, M.$$b5
000018271 7001_ $$0P:(DE-HGF)0$$aJanek, J.$$b6
000018271 773__ $$0PERI:(DE-600)1476244-4$$a10.1039/c003991h$$gVol. 13, p. 1239 - 1242$$p1239 - 1242$$q13<1239 - 1242$$tPhysical Chemistry Chemical Physics$$v13$$x1463-9076$$y2011
000018271 8567_ $$uhttp://dx.doi.org/10.1039/c003991h
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