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000018310 084__ $$2WoS$$aPhysics, Condensed Matter
000018310 1001_ $$0P:(DE-HGF)0$$aLéon, A.$$b0
000018310 245__ $$aHydrogen Release from Sodium Alanate Observed by Time-resolved Neutron Backscattering
000018310 260__ $$aBristol$$bIOP Publ.$$c2011
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000018310 520__ $$aInnermolecular motion in Na(3)AlH(6) gives rise to a Lorentzian spectrum with a wavenumber-independent width of about 1  µeV at 180 °C, which is probably due to the rotation of AlH(6) tetrahedra. There is no such quasielastic line in NaAlH(4) or NaH. Based on this finding, time-resolved measurements on the neutron backscattering spectrometer SPHERES were used to monitor the decomposition kinetics of sodium alanate, [Formula: see text] NaH. Both reaction steps were found to be accelerated by autocatalysis, most likely at the surfaces of Na(3)AlH(6) and NaH crystallites.
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000018310 7001_ $$0P:(DE-Juel1)131044$$aWuttke, J.$$b1$$uFZJ
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000018310 8567_ $$uhttp://dx.doi.org/10.1088/0953-8984/23/25/254214
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